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2,780 Matching Results
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Development of nanostructured and surface modified semiconductors for hybrid organic-inorganic solar cells.
Solar energy conversion is increasingly being recognized as one of the principal ways to meet future energy needs without causing detrimental environmental impact. Hybrid organic-inorganic solar cells (SCs) are attracting particular interest due to the potential for low cost manufacturing and for use in new applications, such as consumer electronics, architectural integration and light-weight sensors. Key materials advantages of these next generation SCs over conventional semiconductor SCs are in design opportunities--since the different functions of the SCs are carried out by different materials, there are greater materials choices for producing optimized structures. In this project, we explore the hybrid organic-inorganic solar cell system that consists of oxide, primarily ZnO, nanostructures as the electron transporter and poly-(3-hexylthiophene) (P3HT) as the light-absorber and hole transporter. It builds on our capabilities in the solution synthesis of nanostructured semiconducting oxide arrays to this photovoltaic (PV) technology. The three challenges in this hybrid material system for solar applications are (1) achieving inorganic nanostructures with critical spacing that matches the exciton diffusion in the polymer, {approx} 10 nm, (2) infiltrating the polymer completely into the dense nanostructure arrays, and (3) optimizing the interfacial properties to facilitate efficient charge transfer. We have gained an understanding and control …
Date:
September 1, 2008
Creator:
Hsu, Julia, W. P.
Object Type:
Report
System:
The UNT Digital Library
Where do fossil fuel carbon dioxide emissions from California go? An analysis based on radiocarbon observations and an atmospheric transport model
Characterizing flow patterns and mixing of fossil fuel-derived CO{sub 2} is important for effectively using atmospheric measurements to constrain emissions inventories. Here we used measurements and a model of atmospheric radiocarbon ({sup 14}C) to investigate the distribution and fluxes of atmospheric fossil fuel CO{sub 2} across the state of California. We sampled {sup 14}C in annual C{sub 3} grasses at 128 sites and used these measurements to test a regional model that simulated anthropogenic and ecosystem CO{sub 2} fluxes, transport in the atmosphere, and the resulting {sup 14}C of annual grasses ({Delta}{sub g}). Average measured {Delta}{sub g} in Los Angeles, San Francisco, the Central Valley, and the North Coast were 27.7 {+-} 20.0, 44.0 {+-} 10.9, 48.7 {+-} 1.9, and 59.9 {+-} 2.5{per_thousand}, respectively, during the 2004-2005 growing season. Model predictions reproduced regional patterns reasonably well, with estimates of 27.6 {+-} 2.4, 39.4 {+-} 3.9, 46.8 {+-} 3.0, and 59.3 {+-} 0.2{per_thousand} for these same regions and corresponding to fossil fuel CO{sub 2} mixing ratios (Cf) of 13.7, 6.1, 4.8, and 0.3 ppm. {Delta}{sub g} spatial heterogeneity in Los Angeles and San Francisco was higher in the measurements than in the predictions, probably from insufficient spatial resolution in the fossil …
Date:
May 1, 2008
Creator:
Riley, W. J.; Hsueh, D. Y.; Randerson, J. T.; Fischer, M. L.; Hatch, J. G.; Pataki, D. E. et al.
Object Type:
Article
System:
The UNT Digital Library
Save Energy Now Reveals New Opportunities for Steel Manufacturers to Reduce Costs and Energy Use
This case study describes how the Industrial Technologies Program helps steel companies find ways to improve the efficiency of energy-intensive process heating and steam systems by performing Save Energy Now energy assessments.
Date:
August 1, 2008
Creator:
unknown
Object Type:
Report
System:
The UNT Digital Library
THE COMPONENT TEST FACILITY – A NATIONAL USER FACILITY FOR TESTING OF HIGH TEMPERATURE GAS-COOLED REACTOR (HTGR) COMPONENTS AND SYSTEMS
The Next Generation Nuclear Plant (NGNP) and other High-Temperature Gas-cooled Reactor (HTGR) Projects require research, development, design, construction, and operation of a nuclear plant intended for both high-efficiency electricity production and high-temperature industrial applications, including hydrogen production. During the life cycle stages of an HTGR, plant systems, structures and components (SSCs) will be developed to support this reactor technology. To mitigate technical, schedule, and project risk associated with development of these SSCs, a large-scale test facility is required to support design verification and qualification prior to operational implementation. As a full-scale helium test facility, the Component Test facility (CTF) will provide prototype testing and qualification of heat transfer system components (e.g., Intermediate Heat Exchanger, valves, hot gas ducts), reactor internals, and hydrogen generation processing. It will perform confirmation tests for large-scale effects, validate component performance requirements, perform transient effects tests, and provide production demonstration of hydrogen and other high-temperature applications. Sponsored wholly or in part by the U.S. Department of Energy, the CTF will support NGNP and will also act as a National User Facility to support worldwide development of High-Temperature Gas-cooled Reactor technologies.
Date:
September 1, 2008
Creator:
Duncan, David S.; Balls, Vondell J. & Austad, Stephanie L.
Object Type:
Article
System:
The UNT Digital Library
THE PRODUCTION OF SYNGAS VIA HIGH TEMPERATURE ELECTROLYSIS AND BIO-MASS GASIFICATION
A process model of syngas production using high temperature electrolysis and biomass gasification is presented. Process heat from the biomass gasifier is used to improve the hydrogen production efficiency of the steam electrolysis process. Hydrogen from electrolysis allows a high utilization of the biomass carbon for syngas production. Based on the gasifier temperature, 94% to 95% of the carbon in the biomass becomes carbon monoxide in the syngas (carbon dioxide and hydrogen). Assuming the thermal efficiency of the power cycle for electricity generation is 50%, (as expected from GEN IV nuclear reactors), the syngas production efficiency ranges from 70% to 73% as the gasifier temperature decreases from 1900 K to 1500 K.
Date:
November 1, 2008
Creator:
McKellar, M. G.; Hawkes, G. L. & O'Brien, J. E.
Object Type:
Article
System:
The UNT Digital Library
Searches for Large Extra Dimensions at the Tevatron
None
Date:
July 1, 2008
Creator:
Krutelyov, Vyacheslav
Object Type:
Article
System:
The UNT Digital Library
Washington International Renewable Energy Conference 2008 Pledges: Methodology and Assumptions Summary
The 2008 Washington International Renewable Energy Conference (WIREC) was held in Washington, D.C., from March 4-6, 2008, and involved nearly 9,000 people from 125 countries. The event brought together worldwide leaders in renewable energy (RE) from governments, international organizations, nongovernmental organizations, and the private sector to discuss the role that renewables can play in alleviating poverty, growing economies, and passing on a healthy planet to future generations. The conference concluded with more than 140 governments, international organizations, and private-sector representatives pledging to advance the uptake of renewable energy. The U.S. government authorized the National Renewable Energy Laboratory (NREL) to estimate the carbon dioxide (CO2) savings that would result from the pledges made at the 2008 conference. This report describes the methodology and assumptions used by NREL in quantifying the potential CO2 reductions derived from those pledges.
Date:
August 1, 2008
Creator:
Babiuch, B.; Bilello, D. E.; Cowlin, S. C.; Mann, M. & Wise, A.
Object Type:
Report
System:
The UNT Digital Library
Assessment of Unabated Facility Emission Potentials for Evaluating Airborne Radionuclide Monitoring Requirements at Pacific Northwest National Laboratory - 2007
Assessments were performed to evaluate compliance with the airborne radionuclide emission monitoring requirements in the National Emission Standards for Hazardous Air Pollutants (NESHAP – U.S. Code of Federal Regulations, Title 40, Part 61, Subpart H) and Washington Administrative Code (WAC) 246-247: Radiation Protection – Air Emissions. In these NESHAP assessments, potential unabated offsite doses were evaluated for emission locations at buildings that are part of the consolidated laboratory campus of the Pacific Northwest National Laboratory. This report describes the inventory-based methods and provides the results for the NESHAP assessment performed in 2007.
Date:
January 1, 2008
Creator:
Ballinger, Marcel Y.; Barfuss, Brad C. & Gervais, Todd L.
Object Type:
Report
System:
The UNT Digital Library
Investigation of the amorphous to crystalline phase transition of chemical solution deposited Pb(Zr30Ti70)O3 thin films by soft x-ray absorption and soft x-ray emission spectroscopy
Chemical solution deposited (CSD) complex oxide thin films attract considerable interest in various emerging fields as for example, fuel cells, ferroelectric random access memories or coated conductors. In the present paper the results of soft-x-ray spectroscopy between 100 eV and 500 eV on the amorphous to crystalline phase transition of ferroelectric PbZr{sub 0.3}Ti{sub 0.7}O{sub 3} (PZT) thin films are presented. Five CSD samples derived from the same wafer coated with a PZT film pyrolyzed at 350 C were heat treated at different temperatures between 400 C and 700 C. At first the sample were morphologically and electrically characterized. Subsequently the soft-x-ray absorption and emission experiments were performed at the undulator beamline 8.0 of the Advanced Light Source of the Lawrence Berkeley National Laboratory. Soft-x-ray absorption spectra were acquired for the Ti L{sub 2,3-}, O K-, and C K-edge thresholds by using simultaneously the total electron yield (TEY) and total fluorescence yield (TFY) detection methods. For two samples, annealed at 400 C and 700 C, respectively, the resonant inelastic soft-x-ray spectroscopy (RIXS) was applied for various excitation energies near the Ti L-, O K-edges. We observed clear evidence of a rutile phase at untypically low temperatures. This rutile phase transforms into …
Date:
August 1, 2008
Creator:
Schneller, T.; Schneller, T.; Kohlstedt, H.; Petraru, A.; Waser, R.; Guo, J. et al.
Object Type:
Article
System:
The UNT Digital Library
Investigation of possible csr induced energy spread effects with the A0 photoinjector bunch compressor
The bunch compressor of the A0 Photoinjector at Fermilab was removed this past spring to install a transverse to longitudinal emittance exchange experiment. Prior to its removal questions arose about the possibility of observing the effects of Coherent Synchrotron Radiation on the compressed beam. The energy spread of the beam with and without compression was measured to observe any changes. Various beam charges were used to look for square law effects associated with CSR. No direct observation of CSR in the compressor was attempted because the design of the vacuum chamber did not allow it. In this paper we report the results of these experiments and comparison with simulations using ASTRA and CSRTrack. The results are also compared with analytical approximations.
Date:
June 1, 2008
Creator:
Edwards, H.; Kazakevich, G.; Thurman-Keup, R. M. & Ruan, J.
Object Type:
Article
System:
The UNT Digital Library
Electrical Contacts to Individual Colloidal Semiconductor Nanorods
We report the results of charge transport studies on single CdTe nanocrystals contacted via evaporated Pd electrodes. Device charging energy, E{sub c}, monitored as a function of electrode separation drops suddenly at separations below {approx}55 nm. This drop can be explained by chemical changes induced by the metal electrodes. This explanation is corroborated by ensemble X-Ray photoelectron spectroscopy (XPS) studies of CdTe films as well as single particle measurements by transmission electron microscopy (TEM) and energy dispersive X-Rays (EDX). Similar to robust optical behavior obtained when Nanocrystals are coated with a protective shell, we find that a protective SiO2 layer deposited between the nanocrystal and the electrode prevents interface reactions and an associated drop in E{sub c,max}. This observation of interface reactivity and its effect on electrical properties has important implications for the integration of nanocrystals into conventional fabrication techniques and may enable novel nano-materials.
Date:
April 1, 2008
Creator:
Trudeau, Paul-Emile; Sheldon, Matt; Altoe, Virginia & Alivisatos, A. Paul
Object Type:
Article
System:
The UNT Digital Library
The Sloan Bright Arcs Survey : Six Strongly Lensed Galaxies at z=0.4-1.4
We present new results of our program to systematically search for strongly lensed galaxies in the Sloan Digital Sky Survey (SDSS) imaging data. In this study six strong lens systems are presented which we have confirmed with followup spectroscopy and imaging using the 3.5m telescope at the Apache Point Observatory. Preliminary mass models indicate that the lenses are group-scale systems with velocity dispersions ranging from 466?878 km s{sup -1} at z = 0.17-0.45 which are strongly lensing source galaxies at z = 0.4-1.4. Galaxy groups are a relatively new mass scale just beginning to be probed with strong lensing. Our sample of lenses roughly doubles the confirmed number of group-scale lenses in the SDSS and complements ongoing strong lens searches in other imaging surveys such as the CFHTLS (Cabanac et al. 2007). As our arcs were discovered in the SDSS imaging data they are all bright (r {approx_equal} 22), making them ideally suited for detailed follow-up studies.
Date:
December 1, 2008
Creator:
Kubo, Jeffrey M.; Allam, Sahar S.; Annis, James; Buckley-Geer, Elizabeth J.; Diehl, H. Thomas; Kubik, Donna et al.
Object Type:
Article
System:
The UNT Digital Library
Fabrication Flaw Density and Distribution In Repairs to Reactor Pressure Vessel and Piping Welds
The Pacific Northwest National Laboratory is developing a generalized fabrication flaw distribution for the population of nuclear reactor pressure vessels and for piping welds in U.S. operating reactors. The purpose of the generalized flaw distribution is to predict component-specific flaw densities. The estimates of fabrication flaws are intended for use in fracture mechanics structural integrity assessments. Structural integrity assessments, such as estimating the frequency of loss-of-coolant accidents, are performed by computer codes that require, as input, accurate estimates of flaw densities. Welds from four different reactor pressure vessels and a collection of archived pipes have been studied to develop empirical estimates of fabrication flaw densities. This report describes the fabrication flaw distribution and characterization in the repair weld metal of vessels and piping. This work indicates that large flaws occur in these repairs. These results show that repair flaws are complex in composition and sometimes include cracks on the ends of the repair cavities. Parametric analysis using an exponential fit is performed on the data. The relevance of construction records is established for describing fabrication processes and product forms. An analysis of these records shows there was a significant change in repair frequency over the years when these components were …
Date:
April 1, 2008
Creator:
Schuster, G. J.; Simonen, F. A. & Doctor, S. R.
Object Type:
Report
System:
The UNT Digital Library
Multi-Component Dark Matter
We explore multi-component dark matter models where the dark sector consists of multiple stable states with different mass scales, and dark forces coupling these states further enrich the dynamics. The multi-component nature of the dark matter naturally arises in supersymmetric models, where both R parity and an additional symmetry, such as a Z{sub 2}, is preserved. We focus on a particular model where the heavier component of dark matter carries lepton number and annihilates mostly to leptons. The heavier component, which is essentially a sterile neutrino, naturally explains the PAMELA, ATIC and synchrotron signals, without an excess in antiprotons which typically mars other models of weak scale dark matter. The lighter component, which may have a mass from a GeV to a TeV, may explain the DAMA signal, and may be visible in low threshold runs of CDMS and XENON, which search for light dark matter.
Date:
November 1, 2008
Creator:
Zurek, Kathryn M.
Object Type:
Article
System:
The UNT Digital Library
Linearly Scaling 3D Fragment Method for Large-Scale Electronic Structure Calculations
We present a new linearly scaling three-dimensional fragment (LS3DF) method for large scale ab initio electronic structure calculations. LS3DF is based on a divide-and-conquer approach, which incorporates a novel patching scheme that effectively cancels out the artificial boundary effects due to the subdivision of the system. As a consequence, the LS3DF program yields essentially the same results as direct density functional theory (DFT) calculations. The fragments of the LS3DF algorithm can be calculated separately with different groups of processors. This leads to almost perfect parallelization on tens of thousands of processors. After code optimization, we were able to achieve 35.1 Tflop/s, which is 39percent of the theoretical speed on 17,280 Cray XT4 processor cores. Our 13,824-atom ZnTeO alloy calculation runs 400 times faster than a direct DFTcalculation, even presuming that the direct DFT calculation can scale well up to 17,280 processor cores. These results demonstrate the applicability of the LS3DF method to material simulations, the advantage of using linearly scaling algorithms over conventional O(N3) methods, and the potential for petascale computation using the LS3DF method.
Date:
July 1, 2008
Creator:
Wang, Lin-Wang; Lee, Byounghak; Shan, Hongzhang; Zhao, Zhengji; Meza, Juan; Strohmaier, Erich et al.
Object Type:
Article
System:
The UNT Digital Library
Survey of Dynamic Simulation Programs for Nuclear Fuel Reprocessing
The absence of any industrial scale nuclear fuel reprocessing in the U.S. has precluded the necessary driver for developing the advanced simulation capability now prevalent in so many other industries. Modeling programs to simulate the dynamic behavior of nuclear fuel separations and processing were originally developed to support the US government’s mission of weapons production and defense fuel recovery. Consequently there has been little effort is the US devoted towards improving this specific process simulation capability during the last two or three decades. More recent work has been focused on elucidating chemical thermodynamics and developing better models of predicting equilibrium in actinide solvent extraction systems. These equilibrium models have been used to augment flowsheet development and testing primarily at laboratory scales. The development of more robust and complete process models has not kept pace with the vast improvements in computational power and user interface and is significantly behind simulation capability in other chemical processing and separation fields.
Date:
June 1, 2008
Creator:
Tranter, Troy J. & Haefner, Daryl R.
Object Type:
Report
System:
The UNT Digital Library
Mixing and CP Violation at the Tevatron
Measurements of meson mixing and CP violation parameters obtained by the CDF and D0 experiments at the Fermilab Tevatron are presented. These include results on B{sub s} and D meson mixing, and searches for CP violation in the decay B{sup +} {yields} J/{psi}K{sup +}, in mixing through semileptonic B{sub s} meson decays, and in the interference between mixing and decay in the process B{sub s} {yields} J/{psi}{phi}.
Date:
August 1, 2008
Creator:
Brooijmans, G.
Object Type:
Article
System:
The UNT Digital Library
INL Site Executable Plan for Energy and Transportation Fuels Management
It is the policy of the Department of Energy (DOE) that sustainable energy and transportation fuels management will be integrated into DOE operations to meet obligations under Executive Order (EO) 13423 "Strengthening Federal Environmental, Energy, and Transportation Management," the Instructions for Implementation of EO 13423, as well as Guidance Documents issued in accordance thereto and any modifcations or amendments that may be issued from time to time. In furtherance of this obligation, DOE established strategic performance-based energy and transportation fuels goals and strategies through the Transformational Energy Action Management (TEAM) Initiative, which were incorporated into DOE Order 430.2B "Departmental Energy, Renewable energy, and Transportation Management" and were also identified in DOE Order 450.1A, "Environmental Protection Program." These goals and accompanying strategies are to be implemented by DOE sites through the integration of energy and transportation fuels management into site Environmental Management Systems (EMS).
Date:
November 1, 2008
Creator:
Fossum, Ernest L.
Object Type:
Report
System:
The UNT Digital Library
Geometric optimization of the 56 MHz SRF cavity and its frequency table
It is essential to know the frequency of a Superconducting Radio Frequency (SRF) cavity at its 'just being fabricated' stage because frequency is the key parameter in constructing the cavity. In this paper, we report our work on assessing it. We can estimate the frequency change from stage to stage theoretically and/or by simulation. At the operating stage, the frequency can be calculated accurately, and, from this value, we obtain the frequencies at other stages. They are listed in a table that serves to check the processes from stage to stage. Equally important is optimizing the geometric shape of the SRF cavity so that the peak electric-field and peak magnetic-field are as low as possible. It is particularly desirable in the 56MHz SRF cavity of RHIC to maximize the frequency sensitivity of the slow tuner. After undertaking such optimization, our resultant peak electric-field is only 44.1MV/m, and the peak magnetic-field is 1049G at 2.5MV of voltage across the cavity gap. To quench superconductivity in an SRF cavity, it is reported that the limit of the peak magnetic-field is 1800G [1], and that of the peak electric-field is more than l00MV/m for a SRF cavity [2]. Our simulations employed the codes …
Date:
October 1, 2008
Creator:
Chang, X. & Ben-Zvi, Ilan
Object Type:
Report
System:
The UNT Digital Library
Intrinsic DX Centers in Ternary Chalcopyrite Semiconductors
The conclusions of this report are: (1) intrinsic donor-type defects In{sub Cu}, Ga{sub Cu}, and V{sub Se}, and their complexes with V{sub Cu} cause metastability, but also act to limit V{sub OC}; (2) growth conditions which minimize these defects (Cu-rich/Se-rich) are very different from those currently used; and (3) overcoming V{sub OC} limitation requires to address other issues and trade-offs.
Date:
May 1, 2008
Creator:
Lany, S. & Zunger, A.
Object Type:
Presentation
System:
The UNT Digital Library
Help for the Developers of Control System Cyber Security Standards
A Catalog of Control Systems Security: Recommendations for Standards Developers (Catalog), aimed at assisting organizations to facilitate the development and implementation of control system cyber security standards, has been developed. This catalog contains requirements that can help protect control systems from cyber attacks and can be applied to the Critical Infrastructures and Key Resources of the United States and other nations. The requirements contained in the catalog are a compilation of practices or various industry bodies used to increase the security of control systems from both physical and cyber attacks. They should be viewed as a collection of recommendations to be considered and judiciously employed, as appropriate, when reviewing and developing cyber security standards for control systems. The recommendations in the Catalog are intended to be broad enough to provide any industry using control systems the flexibility needed to develop sound cyber security standards specific to their individual security requirements.
Date:
May 1, 2008
Creator:
Evans, Robert P.
Object Type:
Article
System:
The UNT Digital Library
The Reactivity and Structural Dynamics of Supported Metal Nanoclusters Using Electron Microscopy, in situ X-Ray Spectroscopy, Electronic Structure Theories, and Molecular Dynamics Simulations.
The distinguishing feature of our collaborative program of study is the focus it brings to emergent phenomena originating from the unique structural/electronic environments found in nanoscale materials. We exploit and develop frontier methods of atomic-scale materials characterization based on electron microscopy (Yang) and synchrotron X-ray absorption spectroscopy (Frenkel) that are in turn coupled innately with advanced first principles theory and methods of computational modeling (Johnson). In the past year we have made significant experimental advances that have led to important new understandings of the structural dynamics of what are unquestionably the most important classes of heterogeneous catalysts—the materials used to both produce and mitigate the consequences of the use of liquid hydrocarbon fuels.
Date:
July 1, 2008
Creator:
Yang, Judith C. & Ralph G. Nuzzo, Duane Johnson, Anatoly Frenkel
Object Type:
Report
System:
The UNT Digital Library
Silicon Solar Cells with Front Hetero-contact and Aluminum Alloy Back Junction (Poster)
The objectives of this report are: (1) to apply industrial back Al process in efficient n-wafer cells with a-Si:H front surface passivation; and (2) to evaluate the surface recombination velocity (SRV) of the a-Si:H passivated front surface with different surface preparation procedures.
Date:
May 1, 2008
Creator:
Yuan, H.-C.; Page, M. R.; Iwaniczko, E.; Xu, Y.; Roybal, L.; Wang, Q. et al.
Object Type:
Article
System:
The UNT Digital Library
Studying neutrino oscillations using quasi-elastic events in MINOS
MINOS (Main Injector Neutrino Oscillation Search), is a long baseline neutrino experiment designed to search for neutrino oscillations using two detectors at Fermi National Accelerator Laboratory, IL (Near Detector) and Soudan, MN (Far Detector). It will study {nu}{sub {mu}} {yields} {nu}{sub {tau}} oscillations and make a measurement on the oscillation parameters, {Delta}m{sub 23}{sup 2} and sin{sup 2} 2{theta}{sub 23}, via a {nu}{sub {mu}} beam made at Fermilab. Charge current neutrino interactions in the MINOS detectors are of three types: quasi-elastic scattering (QEL), resonance scattering (RES) and deep inelastic scattering (DIS). Of these, quasi-elastic scattering leaves the cleanest signal with just one {mu} and one proton in the final state, thus rendering the reconstruction of the neutrino energy more accurate. This thesis will outline a method to separate QEL events from the others in the two detectors and perform a calculation of {Delta}m{sub 23}{sup 2} and sin{sup 2} 2{theta}{sub 23} using those events. The period under consideration was May 2005 to February 2006. The number of observed quasi-elastic events with energies below 10 GeV was 29, where the expected number was 60 {+-} 3. A fit to the energy distribution of these events gives {Delta}m{sub 23}{sup 2} = 2.91{sub -0.53}{sup +0.49}(stat){sub …
Date:
February 1, 2008
Creator:
Kumaratunga, Sujeewa Terasita
Object Type:
Thesis or Dissertation
System:
The UNT Digital Library