This report summarizes the work done to date on the application of the TRUEX solvent extraction process for removing and separately recovering plutonium and americium from a nitric acid waste solution containing these elements, uranium, and a complement of inert metal ions. This simulated waste stream is typical of a raffinate from a tributyl phosphate (TBP)-based solvent extraction process for removing uranium and plutonium from dissolved plutonium-containing metallurgical scrap. The TRUEX process solvent in these experiments was a solution of TBP and octyl(phenyl)-N,N-diisobutylcarbamoylmethylphosphine oxide (CMPO) dissolved in carbon tetrachloride. A flowsheet was designed on the basis of measured batch distribution ratios to reduce the TRU content of the solidified raffinate to less than or equal to 10 nCi/g and was tested in a countercurrent experiment performed in a 14-stage Argonne-model centrifugal contractor. The process solvent was recycled without cleanup. An unexpectedly high evaporative loss of CCl4 resulted in concentration of the active extractant, CMPO, to nearly 0.30M in the solvent. Results are consistent with this higher CMPO concentration. The raffinate contained only 2 nCi/g of TRU, but the higher CMPO concentration resulted in reduced effectiveness in the stripping of americium from the solvent. Conditions can be easily adjusted to give …

Fluid forces are important in the assessment of vibration of the Space Shuttle Main Engine liquid oxygen posts. This report summarizes the available data on fluid excitation forces acting on tube arrays in turbulent crossflow, and test results for an array of tubes subject to turbulent flow. The fluctuating drag and lift forces are measured as a function of Reynolds number, incoming flow conditions, and tube location in an array.

A general theory of fluid-elastic instability for a tube array in crossflow is presented for application to the space shuttle main engine liquid oxygen (SSME LOX) posts. Various techniques to obtain the motion-dependent fluid-force coefficients are discussed and the general instability characteristics are summarized. The theory is also used to evaluate the results of other mathematical models for crossflow-induced instability.

Report of the activities of the physics division at Argonne including the successful completion of Argonne Tandem-Linac Accelerator System.