This report is a progress report detailing operations and ongoing projects at the Brookhaven National Laboratory. The report describes new developments with buildings and progress regarding ongoing experiments. The report includes photographs showing progress in the construction of the reactor and other images and figures that accompany the descriptions of projects.

This technical report discusses techniques that have been developed for "computing the angular thermal flux spectrum emerging from a lattice. These methods are applied to water lattices and it is found that the computed spectra are sensitive to the geometrical description of the lattice, but insensitive to the anisotropic scattering by water. Comparisons with measured spectra indicate that corrections for gradients and the finite size of the experimental lattice are important." -- from abstract (p. 3).

From Abstract: "The diffusion cooling coefficient in graphite has been determined by measuring the change in the asymptotic average velocity with buckling, by pulsed neutron methods. The times necessary to establish equilibrium spectra in graphite and heavy water have been measured and are reported."

From summary: "During 1951 NDA has, at the request of ORNL, been studying the supercritical-water reactor as proposed for aircraft propulsion in Wash-24...This study has concerned itself only with the reactor and shield." The report describes the reactor and the processes involved in developing it. The goal of the development of this reactor is identified as a path to supersonic flight.

The work of the BNL Waste Processing Development Project has been concerned with developing means to accomplish three main objectives in handling radiochemical wastes. One is to reduce the corrosiveness of the waste. At present some wastes must be stored in SS vessels at high cost, since other tankage would not resist corrosion for any length of time. Hanford has solved a part of this problem by storing a neutralized or alkaline waste which can be contained more cheaply in 1020 steel vessels, although neutralization increases its total volume 50 percent over the original acid solution volume. Another aim in waste disposal is to reduce the mobility of the water. Although equipment is checked and double checked, and corrosion resistance is assured by extra thick-walled vessels, the possibility exists that a leak in such storage tanks may develop. At such times the solution may be carried by ground water into populated areas, whereas a relatively immobile waste would remain a local problem. A third and very important consideration is a desirable reduction in total waste volume. Since costs of waste storage are propositional to the volume stored, any reduction in total volume will reduce the total cost.

The biological evaluation of the thermal neutron capture reaction of boron-10, B10 (n,α)Li7 + 2.786 MeV, has previously been studied, using different particles from the boron-10 thermal neutron capture reaction compared with 250 kvp x-rays has been reported as 1.05 for spleen-thymic weight reduction (1), as 1.5 to 2.0 for skin lesions in pigs (2), and 1.87 for skin lesions of the rabbit's ear (3). The significance of such a calculation is felt to be unreliable for the boron-10 reaction in animals because of the vagaries of dose determination resulting from irregular boron distribution, and by the presence of an adventitious irradiation from fast neutrons and capture gammas that is inadequately determined at present. Our present experiment attempts to circumvent the difficulties attendent to studies of the boron-10 reaction in animals by comparing the effect of this reaction on the proliferative capacity of HeLa cells with those produced with 250 kvp x-ray.

In these lectures we will discuss some examples of information about magnetic properties of solids which can be obtained by neutron scattering. We consider a scattering process in which a neutron with wave vector k and spin σ is incident upon a solid in state q>. (Here q stands for all of the quantum numbers which describe the state of the solid, such as spin and orbital electronic states, phonon numbers, etc.) After interacting with the solid, the neutron goes off with wave-vector k' and spin σ', leaving the solid in state q'>. In performing an experiment of this sort one does not usually observe the initial and final spin states of the neutron or the initial and final states of the solid. We must then sum over all possible final states and average over all initial states.

We consider the kinetic isotope effect in three center reactions of the type of A+BC→AB+C. Such model calculations are a good approximation to primary hydrogen isotope effects. For abstraction or transfer reactions, B becomes H, D, or T. The dynamics of the three storm system are calculated for a general quadratic potential, with the assumption that the potential energy is constant along the reaction coordinate (flat top barrier). This model system can be calculated in detail and serves to illustrate the relationship between kinetic isotope effect and chemical bonding in the transition state. The statistical mechanical part of the calculation can be carried out exactly within the framework transition state theory or in any one of a number of approximations. The γ bar method gives particularly good insight into the chemistry of the problem with a minimum of arithmetic.

Optical absorption and photoconductivity measurements have been made on single crystals of pure synthetic rutile (TiO2). Reactor irradiations at 70°C totaling 4.8 x 10 18 nvt fast and 1.69 x10 19 nvt slow did not produce any discernible optical absorption bands; however, the transmission decreased 5 percent at all wavelengths. Reactor irradiation induced a [illegible] five photoconduction peaks in the wavelength range 4200 to 14,000 A. In addition the photopeak at 4065 A (3.05 eV) was enhanced and there were drastic changes in the dependence of photocurrent with light intensity. Gamma-ray irradiations as large as 10 9 r do not change the conduction properties. The photocurrent is proportional to a power of the light intensity; the power range from 0.65 to 1.24, for the crystals described in this work. The photocurrent vs. voltage dependence is more complex.

The present core of the Brookhaven Graphite Reactor consists of some 4900 highly enriched uranium fuel loaded in 615 horizontal fuel channels passing through a 25 foot cube of graphite moderator and reflector. The core is divided into two halves (north and south) by an 8 cm. wide vertical gap in the center of the graphite. The cooling air enters the reactor through inlet filters, at the rate of 270,000 CFM, passes into the central gap and flows bi-directionally through the north and south halves of the core. It then enters the collecting plenums and flows into the north and south ducts. The air is first monitored by the north and south exit air monitors located within the pile building. These are moving filter tape monitors with beta scintillation detectors. They are essentially operational monitors and are maintained by reactor operations. They are essentially operational monitors and are maintained by a reactor operations. The air then passes through the exit air filters, heat exchanger, venturi and on to the fan house where the north and south ducts join. After the fan house the air is monitored by Argon-41 by a Kanne ion chamber syste.

Boron-10 has a high thermal neutron capture cross section (3880 barns). Following neutron capture, the subsequent nuclear disintegration produces an alpha particle and a lithium-7 nucleus with the release of an average of 2.34 MeV for the particle irradiation, and in 93% of the reactions there is also the emission of an 0.48 MeV gamma ray: [equation not transcribed]. The kinetic energy is divided between the lithium-7 nucleus and the alpha particle giving the equal and opposite momentums with a range in tissue of about 8-14μ or approximately 1 cell diameter (1). This fact and the reported favorable partition of boron between tumor and the normal brain suggested a possible therapeutic usefulness which has been investigated clinically. The object of our study is to document the biological effects of the B10 (n,α) Li7 reaction on the brain of dogs injected with boron-10 30 minutes prior to irradiation with thermal neutrons. For this, we felt it desirable to estimate a dose for the boron-10 reaction which if exceeded, produces destruction of normal tissue. This dose could then be a reference dose to be utilized as a maximal limit for the irradiation of normal tissue. We have assured that the largest fluence …

There is but little known about the thermal process involving the dynamics and thermodynamics of the cycling liquid H2 in the chamber and those of the H2 fluid flow in the cooling coil as well as the geometrical characteristics of the chamber body. This the physical equations governing this process are involving so many variables that this analysis becomes rather complex even if simplifying assumptions are made. To those difficulties is added the ignorance even of an approximative expression for some physical quantities such as film heat transfer coefficients entering as major parameters the process equation.

The purpose of this report is to determine the amount of refrigeration capacity required to cool down the 80" bubble chamber from ambient temperature to liquid hydrogen temperature.

The undercarriage system is required for translating, rotating, and lifting the 450 ton magnet and bubble chamber assemblies so that it can be accurately positioned in the experimental proton beam of the synchrotron. The system must make provision for the two magnet sections to be separated for the purpose of adjustment and maintenance of internal components.

The following general description of the theory and operation of a bubble chamber is presented so that firms who are interested in fabricating components for the Brookhaven 80" chamber will have a better understanding of the design parameters associated with it. This understanding, coupled with the fabricator's knowledge of manufacturing techniques, should enable the fabricators to suggest solutions to manufacturing problems consistent with requirements for chamber operation. In an effort to increase knowledge of fundamental nuclear particles and their interactions at high energies, various types of detecting equipment have been developed. One of these detectors recently developed is the bubble chamber. While there are variations as to liquids used, expansion techniques, means of illumination, etc. the basic concepts upon which all bubble chambers operate are similar. Therefore, it will be sufficient in this report to consider only one specific type, that is a chamber using liquid hydrogen

The analyzer can be operated either internally or externally. The 10 ma germanium discriminator is quiescently biased to 8.5 ma in its low-voltage state. An input signal current of 3.5 ma or more triggers it to its high voltage state. This triggers the oscillator. The oscillator signal is buffered and mixed in the bridge modulator with the reference radiofrequency signal from the cyclotron. The low-frequency beat note from the bridge modulator is squared up and passed to the beat zero univibrator which generates 0.7 mu sec signals each time the beat note passes through zero from positive to negative. The trailing edge of the beat zero univibrator is employed to terminate the time-of-flight measurement and to control the servo measurement. Drawings are included. (M.C.G.)

The problem of separation of beams of particles of different masses but of the same momentum at Bev energies is the subject of a great deal of study at several high energy laboratories. In this note we shall describe the problem and tabulate a few of the cogent parameters. Frequently the student of high energy interactions is faced with a beam of miscellaneous particles coming from an accelerator. By standard techniques this beam can be rendered approximately parallel and an inch or so in diameter. By passage through a magnetic field the beam can be analyzed in momentum. Now it frequently happens that the particles in which the experimenter is particularly interested make up only a small fraction of the beam and the exigencies of the proposed experiment may well demand that the background of undesired particles be drastically reduced. The problem is difficult because the velocities of the various particles are almost equal to each other and to the velocity of lights; this makes time-of-flight techniques relatively ineffective. The energies of the particles are almost equal so electrostatic separation also is difficult. Since the beam is already analyzed in momentum, further separation by magnetic means is impossible.

Nusselt numbers have been calculated for heat transfer to fluids flowing through annuli under conditions of uniform heat flux and fully established velocity and temperature profiles. The following cases were considered: (a) laminar flow, (b) slug flow, (c) turbulent flow with molecular conduction only, and (d) turbulent flow with both molecular and eddy conduction. These Nusselt numbers were determined for two conditions: heat transfer from the inner wall only and heat transfer from the outer wall only. The results were correlated by semi-empirical equations. The final results obtained on cases (a), (b), and (c) are applicable to any fluid, whereas those obtained on (d) are for liquid metals only. Wall- and bulk-temperature relationships for the above four cases were also determined. These relationships were treated as dimensionless temperature ratios. Both the Nusselt numbers and temperature ratios were evaluated over the r1/r2 range, zero to unity; the former being the case of the circular pipe, and the latter, the case of infinite parallel plates.

Internal-conversion coefficients may be thought of as consisting of two parts: a usually dominant part which depends only on the atomic number and the nuclear transition energy, and a usually small part depending explicitly on nuclear transition matrix elements. This latter part arises from the penetration of the converting atomic electrons within the transforming nucleus.

A previous report on this subject (Brookhaven National Laboratory, AGS Internal Report, ECR-4) described in detail the methods of measuring the injected and accelerated proton currents in the Brookhaven AGS up to May 1961. At that time the accelerated current was measured by extracting the bunch frequency component of the signal given by a pair of radial position observation electrodes. The injected current was also determined by the signal induced on a similar pair of radial position electrodes. Absolute values were then determined from machine parameters and a wire measurement of the electrode sensitivities. Linac currents, however, were measured with transformers, calibrated by putting known current pulses through a single turn loop. As described in ECR-4, a crude current transformer was placed on the AGS ring and cross-calibration measurements were carried out using a half turn injected beam. The pickup electrode value was then found to be about 10% higher than that given by the current transformer. This amount of disagreement was within the estimated accuracy of the measurements and calibrations used at that time.

The discovery of the vector meson which mediates the weak interactions, W,1 would be of extreme importance for weak interaction physics and for field theory in general. The W, if it exists, will be made in a variety of processes such as v+N →W+ + e- + N, or n- + P →W- + P, or, as studied in this note, P + P → D + W+. The W couples to leptons with a dimensionless constant [constant not transcribed] where G is the Feral constant defined t=so that [constant not transcribed]. Thus for [equation not transcribed] and the smallness of this constant is, evidently, what makes any of the above processes difficult to detect. The W may have a variety of decay modes.

Report issued by the Brookhaven National Laboratory discussing the instrumentation, operation, and maintenance of the established area radiation monitoring stations. This report includes maps, tables, illustrations, and photographs.

Report issued by the Brookhaven National Laboratory discussing capture positron ratios. As stated on page 1, "the purpose of this report is to present aids for the simple determination of the relative probabilities of K-electron capture and positron emission for allowed and first-forbidden transitions" (p. 1). This report includes tables, and illustrations.

Report issued by the Brookhaven National Laboratory discussing methods of nitrogen fixation, and their economic impacts. As stated in the introduction, "studies are described on circulating dust fuels, as well as fixed plated, porous bed, and other types of fuels as the basis for chemo-nuclear reactor designs, and the various fuel systems are compared on a technical and economic basis" (p. 3). This report includes tables, and illustrations.