Leaching tests were run on two samples from the Grants area in New Mexico. Uranium extractions of 94 per cent were obtained by leaching Sample 6-1 with solutions containing 240 lbs. of Na2CO3 and 60 lbs. of NaHCO3 per ton and by leaching Sample 6-2 with 270 lbs. of Na2CO3 and 180 lbs. of NaHCO3 per ton. Cyclic tests were completed using caustic precipitation of the leach liquor.

The attenuation curve of the deuterons stripped from He3 has been measured with a Faraday cup. The corresponding curve at 190 Mev was fit by assuming that the deuterons were monoenergetic, with three processes taking place.

Removal of particles from air is discussed in terms of three classes of filtering media--air-sampling, respirator, and air-cleaning. Plots of efficiency versus filtering velocity are presented. The pressure drop characteristics of the filters are discussed in terms of initial pressure drops of the clean filters, variations in pressure drop of the individual filters, and comparison of loading rates.

The following report describes polarographic methods that determine saturated aliphatic carbonyl compounds.

Various non-linear calculations for heat conduction in an istropic, homogeneous medium are presented.

Abstract. Samples of pile graphite, irradiated in a test-hole at Hanford for 15 months, have been assayed for radioactive C14, yielding 0.38 ± 0.04 microcuries per gram. At this level of activity, the pile graphite contains very valuable amounts of C14. The relation between the above assay and the probable average assay of pile graphite is discussed, and it is concluded that the latter is almost certainly above 0.3 uc/ gram. Controlled oxidation of this graphite, either with oxygen at ~ 750°C, or with chromic acid "cleaning solution" at room temperature, yields early fractions which are highly enriched in C14. Concentrations of 5-fold with oxygen, and 50-fold with CRO{sub3}, have been observed. The relation between the observed enrichment and the Wigner effect is discussed, and a mechanism accounting for the observations put forward. According to this, about 25% of the stable carbon atoms in the lattice have been displaced by Wigner effect, a large fraction of which have healed the migrating to crystal edges. All the C14 atoms have been displaced, and the same fraction of these migrate to the edges. The enrichment then results from surface oxidation, in the oxygen case. Predictions are made on the basis of this …

Abstract: "The sensitivity to fast neutrons of a CP Meter ionization chamber of the type used for health physics beta and gamma survey measurements has been investigated."

In 1949 Barad presented two solutions to the general diffusion equation. Basic in both solutions is the assumption that in very stable atmospheres a point source may be replaced by a vertical area of uniform concentration at a short distance downwind. This vertical area is considered to exist at the distance at which the plume finally "levels-off" and assumes a flat ribbon-like appearance. In addition if the distance over which diffusion takes place is limited to one or two miles and if only the stable atmosphere with its narrow range of eddy sizes is considered, the average diffusion co-efficient (K) has a signficance which it does not have in the case of neutral equilibrium.

Under the stimulus of electronic materials development - particularly thin-film studies - and the need for space environmental simulation chambers, a very rapid increase in the availability of industrial-sized vacuum components and systems operable in the ultrahigh vacuum range has taken place in the last three years. It is the purpose of this paper to explore the design considerations of ultrahigh vacuum systems for metallurgical applications.

The following report provides tables that measure the pressure of hydrogen fluoride at given temperatures and the hydrolysis of uranium tetrafluoride.

The alternating-gradient proton synchrotrons at CERN and Brookhaven are very similar in size, design and in their experimental use. For this reason, collaboration between the groups at CERN and Brookhaven has been close throughout the history of these two machines. For the most part this has taken the form of exchanges of visits of individual machine designers and of high-energy physicists. By 1962, however, it appeared that the reciprocal flow of information was not adequate and a more formal meeting was arranged. This meeting took place at Brookhaven during the week of September 10, 1962. CERN sent a representative group of machine physicists and high-energy physicists. The meeting was attended also by observers from several American high-energy installations. The discussion covered a wide range of topics, from operating characteristics of the machines themselves to future trends in design of experimental equipment. Plans for beam ejection were presented, techniques were described for better use of secondary beams from internal targets, progress was summarized on dc and rf particle separators. and future trends in neutrino experimentation were predicted.

The purpose of this report is to summarize the work done at KAPL on physical properties of high density concretes.

Report discussing the trajectories of blobs of plasma as it travels across a magnetic field. Various observations are made about the blobs, such as the fact that they are diamagnetic, and that they can be either elastically scattered from each other or form a compound entity with a possible toroidal structure. "It is believed that these blobs are actually stable configurations of plasma and magnetic field, having both diamagnetic moment and spin."

This document is the third in a series of progress report that records investigations of graphite bodies. Along with the report, two appendices are given to describe the different graphite bodies: "Synthetic Binders for Carbon and Graphite" and "High Temperature Physical Properties of Molded Graphites".

The measurement of a alpha-particle energy has been used by many radiochemical laboratories for the identification and analysis of alpha-active radio nuclides. The use of the total-ionization method for alpha-active radio-nuclides. The use of the total-ionization method for alpha energy in ionization chamber in which the alpha particle loses all its energy in ionization of the chamber gas. Collection of the electrons thus formed generates a voltage pulse across the chamber capacity which is proportional to the alpha particle energy. This pulse is then amplified using a suitable linear amplifier and fed to a pulses as to amplitude; the information is then recorded or stored. Since the pulse amplitude is proportional to the alpha energy lost to the chamber gas, the pulse height analysis can be used to estimate the energy of the alpha particles and in the case of several alpha emitters of different energies, the relative abundance of the alpha emitters can be determined. An alpha energy analyzer system using the ion collection method has been fabricated for use in radiochemical laboratories required to perform a large number of alpha energy determinations. This report describes the operation, maintenance, and application of this alpha energy analyzer system.

The general program established at Argonne National Laboratory in connection with the Fast Power Breeder Reactor (PBR) includes performance of exponential experiments on assemblies having compositions which may exist in the reactor core. This report deals with that phase of the program known as the Fast Exponential Experiment which may be described very briefly as follows. An assembly of fissile (U-235) and fertile material (too small to be self-critical) intermixed with poisons (such as are encountered in the mechanical structure and coolant system of a self-sustaining reactor) is fed with neutrons from an auxiliary source. By measurements of the neutron flux within the assembly, important parameters can be calculated which are necessary to the proport design of an actual critical reactor of the same composition.

Abstract: The primary coolant of the SM-1 (APPR-1) was analyzed for short-lived and fission product activities. Manganese-56 was found to be the predominant non-fission product nuclide contributing to the short lived activity. Fission products were found in the coolant. It is concluded these fission products originate from a defects in the cladding and from surface contamination of the fuel elements.

Abstract: The results of activity buildup studies in the SM-1 (APPR-1) performed from February 1958 to January 1959 are reported. Data are presented on the extent, nature, and mechanism of the buildup of long-lived gamma emitting nuclides in the reactor primary system. Mathematical equations to describe the activity buildup are derived. Radiation levels after reactor shutdown are presented, as well as the predicted radiation levels at the end of core life.

From introduction: "The purpose of this report is to summarize some of the observations on the dispersion and rate of disengaging of liquid-liquid systems and suggest some possible lines of future work."

Introduction: "The adoption of aluminum nitrate as salting agent in the Redox process made it imperative that a method be available for determining plutonium in the presence of aluminum. However, large amounts of aluminum have been found to interfere with the determination of plutonium by the lanthanum fluoride procedure. Previous attempts to increase the accuracy of the lanthanum fluoride method, by precipitating LaF3 from 4 M HF (rather than 2 M), have been successful only when the initial plutonium level was high."

A preliminary chemical flowsheet is presented of a fluoride volatility process for recovering and decontaminating uranium from heterogeneous reactor fuels after dissolution in a fused salt. In laboratory work, a gross β decontamination factor of > 10 4 was obtained in the fluorination of a UF4-NaF-ZrF4 melt by passing the product UF6 through NaF at 650°C. The solubility of UF6 in molten NaF-ZrF4 was shown in kinetic studies to cause a lag in the evolution of UF6 from the fluorinator. Corrosion of nickel in the fluorination step appeared to be 2-4 mils/hr during the time that uranium was present. The average corrosion rate over the process as a whole was less than O.4 mil/hr. Earlier studies were reported in ORNL-1709 and 1877.

From Abstract: "The heat treatment and mechanical properties of four zirconium alloys...were investigated. Tensile, hardness, Jominy end-quench, and metallographic data constitute the basis for much of the report. Other data reported include the results of high-temperature creep, tensile, hardness, cold rolling, thermal-cycling, and dynamic-modulus tests." A connection is made between the behavior of these four alloys and more alloys in the zirconium-uranium system.

Objective: The objective of this study is to develop a simple method of either removing the C1- ion from the RAW or converting the ion into a less corrosive valence state.

Thermal oxidation of graphite in flowing CO2 is being studied at 650 to 850 C, in a single-pass gas system at atmospheric pressure, by observing weight loss rates. The method is used to provide comparative data for candidate reactor graphites. The effects on oxidation rates of graphite purity, structure, coke type, graphitization temperatures and other manufacturing variables are determined. In addition, the effects of gas flow rates and graphite surface to volume ratios are observed.