The absolute differential cross sections for elastic scattering of 31-Mev He3 ions on Be, Al, Cu, Sn(nat), Sn120, and Bi have been measured in the angular range of approximately 10 to 120 deg in the center-of-mass system. Thin self-supporting foil targets were chosen to span the parameter A 1/3, where A is the target mass number. The first excited states of the isotopes of the above elements had sufficient energy separation from the ground state to enable elastic scattering to be resolved from inelastic scattering. The detection system, consisting of Cal(Tl) scintillation crystals, was capable of 3%pulse-height resolution and 1 degree angular resolution. Characteristically, the light-element angular distributions show strong diffraction effects. The differential cross section divided by the Rutherford cross section decreases exponentially at large angles for the heavy elements, and the differential cross sections break away from Rutherford behavior at angles which increase almost linearly with increase of atomic number of the target nucleus. A comparison of the results for natural tin, and tin enriched to 85% in Sn120, indicated that within the experimental uncertainties over the measured angular interval, there were no pronounced isotopic effects. The data are presented both in tabular and graphical form to allow …

Annual report describing progress on unclassified research programs funded by the U.S. Atomic Energy Commission during the 1965-66 fiscal year.

Introduction. The phase diagram data reported in this paper were obtained during an investigation of the beryllium-metal compounds of the titanium group transition elements. Several compounds in these systems had been previously reported but their compositions and structures were not all known. In the course of this study many details of the phase diagrams of the system were observed. Tentative diagrams consistent with this data will be presented.

The purpose of this experiment is to study the quantitative adsorption characteristics of a carbon adsorber bed receiving a radioactive inert gas in a helium stream. An objective of the experiment is to measure the equilibrium transmission of the radio-active gas through a carbon adsorber in order to determine if radio-active decay of the adsorbed gas permits additional adsorption.

Tests were conducted to determine the friction factor of randomly packed beds of 3/4-inch diameter spheres in 8-inch and 15-1/4-inch diameter beds, and of 1-1/2-inch diameter spheres in 15-1/4-inch diameter bed. The bed depths were varied in an attempt to isolate the effects of entrance and exit losses. The bed Reynolds number, base on sphere diameter, was varied from 5,000 to 50,000.

Previous studies have been made of the relationship among acceleration, specific power, payload fraction, and travel time for many interplanetary missions. These utilized tangential thrust and correspond to the high thrust Hohmann transfer orbits. In addition, a complete optimization of the one way Mars mission has been accomplished. Since the minimum Jupiter round trip time was six and a half years for tangential thrust, calculations were carried out using higher energy transfer orbits. It is shown that the orbit-matching problem cannot be solved with tangential thrust programming in this case. The initial period of acceleration away from the earth's orbit was accomplished using tangential thrust in order to minimize energy expenditure. This was followed by a period of coasting until the proper moment arrived for commencing the orbit-matching maneuver. This terminates when the velocity and spatial coordinates of Jupiter's orbit are matched. The technique used for accomplishing these various orbit matching conditions without iteration are described. Best results for the final maneuver were obtained with the thrust vector approximately normal to the velocity vector. By this technique it is shown that the round-trip Jupiter mission may be carried out in four and an half years with 16% payload and 0.10 …

"A comparison of the grafting of a 2:1 molar mixture of methacrylic acid and styrene to both polypropylene film and fabric using CO60 source and electron accelerator as sources of ionizing radiation is made on the basis of mutual or simultaneous grafting and post-irradiation grafting.

"Rates of acetylene polymerization induced by Kr/sup 85/ in d-c fields were up to 15 times greater than those observed when no fields were imposed. Work to determine the relations between acetylene pressure, Kr/sup 85/ concentration, and the field intensity is continuing. In other activities, equipment is being designed to study the effects of megacycle electric fields on radioinduced chemical reactions."

""Progress is reported on: design of a continuous flow system for the irradiation of silane using a Cos5 source; pile irradiation of silane samples at elevated temperatures; investigation of materials other than silane, including nonsilicon compounds as well as those containing the silyl group; modification of the existing vacuum system for handling larger quantities of silane as well as increasing the accuracy of the pressure measurements; and use of an electric discharge for the decomposition of silane. Studies were continued on the radiation- and thermalinduced decomposition of sikane at 325 and 350 deg C. A preliminary value of G= 33 was obtained for silane."

"Progress is reported on: design of a continuous flow system for the irradiation of silane using a Cos5 source; pile irradiation of silane samples at elevated temperatures; investigation of materials other than silane, including nonsilicon compounds as well as those containing the silyl group; modification of the existing vacuum system for handling larger quantities of silane as well as increasing the accuracy of the pressure measurements; and use of an electric discharge for the decomposition of silane. The work performed during the period of this report consisted of the following: 1. Preparation of samples of trichlorosilane and hydrogen and subsequent thermal and irradiation studies, and analysis of these samples. 2. Preparation of mixed samples of silane and argon and subsequent thermal and irradiation studies and and analysis. 3. Outlining of future investigations to be conducted on this project."

The chief purpose of this contract is the development of ceramic materials with high dielectric constant and high dielectric strength values, and suitable for use of dielectrics in capacitors capable of storing large amounts of energy in small volumes. Work performed during the fifth quarter included (1) Material development and sample preparation; (2) Sample testing; (3) Optical studies of titanates; (4) Fabrication of large ceramics; and (5) Capacitor design.

The chief purpose of this contract is the development of ceramic materials with high dielectric constant and high dielectric strength values, and suitable for use of dielectrics in capacitors capable of storing large amounts of energy in small volumes. Work performed during the fourth quarter included (1) Material development and sample preparation; (2) Sample testing; (3) discussion of ceramic density measurements; (4) Optical studies of titanates; (5) Fabrication of large ceramics; and (6) Capacitor design.

The objective of this program is the experimental determination of basic physical data and employment of these data to establish and confirm a theoretical model for predicting the long-term changes in isotopic composition and reactivity in plutonium-enriched, light-water-moderated reactors.