Spatiotemporal variations in growing season exchanges of CO2, H2O,and sensible heat in agricultural fields of the Southern GreatPlains (open access)

Spatiotemporal variations in growing season exchanges of CO2, H2O,and sensible heat in agricultural fields of the Southern GreatPlains

Climate, vegetation cover, and management create fine-scaleheterogeneity in unirrigated agricultural regions, with important but notwell-quantified consequences for spatial and temporal variations insurface CO2, water, and heat fluxes. We measured eddy covariance fluxesin seven agricultural fields--comprising winter wheat, pasture, andsorghum--in the U.S. Southern Great Plains (SGP) during the 2001-2003growing seasons. Land-cover was the dominant source of variation insurface fluxes, with 50-100 percent differences between fields planted inwinter-spring versus fields planted in summer. Interannual variation wasdriven mainly by precipitation, which varied more than two-fold betweenyears. Peak aboveground biomass and growing-season net ecosystem exchange(NEE) of CO2 increased in rough proportion to precipitation. Based on apartitioning of gross fluxes with a regression model, ecosystemrespiration increased linearly with gross primary production, but with anoffset that increased near the time of seed production. Because theregression model was designed for well-watered periods, it successfullyretrieved NEE and ecosystem parameters during the peak growing season,and identified periods of moisture limitation during the summer. Insummary, the effects of crop type, land management, and water limitationon carbon, water, and energy fluxes were large. Capturing the controllingfactors in landscape scale models will be necessary to estimate theecological feedbacks to climate and other environmental impactsassociated with changing human needs for agricultural production of …
Date: June 13, 2007
Creator: Fischer, Marc L.; Billesbach, David P.; Berry, Joseph A.; Riley,William J. & Torn, Margaret S.
System: The UNT Digital Library
CHARACTERIZATION OF A HIGH CURRENT INDUCTION ACCELERATOR ELECTRON BEAM VIA OPTICAL TRANSITION RADIATION FROM DIELECTRIC FOILS (open access)

CHARACTERIZATION OF A HIGH CURRENT INDUCTION ACCELERATOR ELECTRON BEAM VIA OPTICAL TRANSITION RADIATION FROM DIELECTRIC FOILS

Traditionally, thin metal foils are employed for optical transition radiation (OTR) beam diagnostics but the possibility of shorting accelerator insulating surfaces and modifying accelerating fields are concerns. The successful utilization of dielectric foils in place of metal ones could alleviate these issues but necessitates more understanding of the OTR data for inferring desired beam parameters because of the dielectric's finite permittivity. Additionally, the temperature dependence of the relevant foil parameters due to beam heating should be accounted for. Here, we present and discuss sample synthetic diagnostic results of Kapton OTR spot-size measurements from the Flash X-Ray (FXR) accelerator which studies these and sightline effects. These simulations show that in some cases, the observed spot-sizes and radii are noticeably larger than the beam radii.
Date: June 13, 2007
Creator: Tang, V; Brown, C & Houck, T
System: The UNT Digital Library
Machine-Detector Interface Issues for the ILCPolarimeters (open access)

Machine-Detector Interface Issues for the ILCPolarimeters

This note examines several Machine-Detector Interface (MDI) issues for the Compton polarimeters in the Beam Delivery System of the International Linear Collider (ILC), including (1) alignment tolerances, (2) impact of crossing angle and IR magnets on spin alignment, (3) Z-pole operation, and (4) costs and conventional facilities.
Date: June 13, 2008
Creator: Woods, Mike
System: The UNT Digital Library
SHOCK INITIATION EXPERIMENTS ON PBX 9501 EXPLOSIVE AT PRESSURES BELOW 3 GPa WITH ASSOCIATED IGNITION AND GROWTH MODELING (open access)

SHOCK INITIATION EXPERIMENTS ON PBX 9501 EXPLOSIVE AT PRESSURES BELOW 3 GPa WITH ASSOCIATED IGNITION AND GROWTH MODELING

Shock initiation experiments on the explosive PBX 9501 (95% HMX, 2.5% estane, and 2.5% nitroplasticizer by weight) were performed at pressures below 3 GPa to obtain in-situ pressure gauge data, run-distance-to-detonation thresholds, and Ignition and Growth modeling parameters. Propellant driven gas guns (101 mm and 155 mm) were utilized to initiate the PBX 9501 explosive with manganin piezoresistive pressure gauge packages placed between sample slices. The run-distance-to-detonation points on the Pop-plot for these experiments showed agreement with previously published data and Ignition and Growth modeling parameters were obtained with a good fit to the experimental data. This parameter set will allow accurate code predictions to be calculated for safety scenarios in the low-pressure regime (below 3 GPa) involving PBX 9501 explosive.
Date: June 13, 2007
Creator: Chidester, S K; Thompson, D G; Vandersall, K S; Idar, D J; Tarver, C M; Garcia, F et al.
System: The UNT Digital Library
DYNAMIC LOADING OF TEFLON AT 200?C (open access)

DYNAMIC LOADING OF TEFLON AT 200?C

Dynamic loading experiments were performed on inert Teflon (Polytetrafluoroethylene) samples, initially heated to the temperature of 200 C, to test its behavior under these conditions for its use in other heated experiments. Tests were performed in the 100 mm diameter bore propellant driven gas gun with piezo-resistive manganin pressure gauges imbedded into the samples to measure loading pressures. Experimental data provided new information on the shock velocity - particle velocity relationship for the heated material and showed no adverse effect of temperature on the insulating properties of the material.
Date: June 13, 2007
Creator: Urtiew, P A; Forbes, J W; Tarver, C M; Vandersall, K S & Garcia, F
System: The UNT Digital Library
The US Support Program to IAEA Safeguards Priority of Containment and Surveillance (open access)

The US Support Program to IAEA Safeguards Priority of Containment and Surveillance

The United States Support Program (USSP) priority for containment and surveillance (US) focuses on maintaining or improving the reliability and cost-effectiveness of C/S systems for IAEA safeguards, expanding the number of systems that are unattended and remotely monitored, and developing verification methods that help streamline the on-site inspection process. Existing IAEA C/S systems have evolved to become complex, integrated systems, which may include active seals, nondestructive assay (NDA) instruments, video cameras, and other sensors. These systems operate autonomously. They send analytical data to IAEA headquarters where it can be reviewed. These systems present challenges to the goals of improved system performance, standardization, reliability, maintainability, documentation, and cost effectiveness. One critical lesson from past experiences is the need for cooperation and common objectives among the IAEA, the developer, and the facility operator, to create a successful, cost effective system. Recent USSP C/S activities include Rokkasho Reprocessing Plant safeguard systems, production of a new shift register, numerous vulnerability assessments of C/S systems, a conduit monitoring system which identifies tampering of IAEA conduit deployed in the field, fiber optic seal upgrades, unattended monitoring system software upgrades, next generation surveillance system which will upgrade existing camera systems, and support of the IAEA's development of …
Date: June 13, 2008
Creator: Diaz,R.A.
System: The UNT Digital Library
A brief review of the intensity of lines 3C and 3D in neon-like Fe XVII (open access)

A brief review of the intensity of lines 3C and 3D in neon-like Fe XVII

X-ray emission from neon-like Fe XVII has been measured with high-resolution spectrometers from laboratory or celestial sources for nearly seven decades. Two of the strongest lines regularly identified in these spectra are the {sup 1}P{sub 1} {yields} {sup 1}S{sub 0} resonance, and {sup 3}D{sub 1} {yields} {sup 1}S{sub 0} intercombination line, known as 3C and 3D, respectively. This paper gives a brief overview of measurements of the intensities of the lines 3C and 3D from laboratory and celestial sources, and their comparison to model calculations, with an emphasis on measurements completed using an electron beam ion trap. It includes a discussion of the measured absolute cross sections compared to results from modern atomic theory calculations, as well as the diagnostic utility of the relative intensity, R = I{sub 3C}/I{sub 3D}, as it applies to the interpretation of spectra measured from the Sun and extra-Solar sources.
Date: June 13, 2007
Creator: Brown, G V
System: The UNT Digital Library
Mechanical Design of the LSST Camera (open access)

Mechanical Design of the LSST Camera

The LSST camera is a tightly packaged, hermetically-sealed system that is cantilevered into the main beam of the LSST telescope. It is comprised of three refractive lenses, on-board storage for five large filters, a high-precision shutter, and a cryostat that houses the 3.2 giga-pixel CCD focal plane along with its support electronics. The physically large optics and focal plane demand large structural elements to support them, but the overall size of the camera and its components must be minimized to reduce impact on the image stability. Also, focal plane and optics motions must be minimized to reduce systematic errors in image reconstruction. Design and analysis for the camera body and cryostat will be detailed.
Date: June 13, 2008
Creator: Nordby, Martin; Bowden, Gordon; Foss, Mike; Guiffre, Gary; Ku, John & Schindler, Rafe
System: The UNT Digital Library
Sequencing and Analysis of Neanderthal Genomic DNA (open access)

Sequencing and Analysis of Neanderthal Genomic DNA

Recovery and analysis of multiple Neanderthal autosomalsequences using a metagenomic approach reveals that modern humans andNeanderthals split ~;400,000 years ago, without significant evidence ofsubsequent admixture.
Date: June 13, 2006
Creator: Noonan, James P.; Coop, Graham; Kudaravalli, Sridhar; Smith,Doug; Krause, Johannes; Alessi, Joe et al.
System: The UNT Digital Library
Chandra Reveals Twin X-ray Jets in the Powerful FR-II Radio Galaxy 3C353 (open access)

Chandra Reveals Twin X-ray Jets in the Powerful FR-II Radio Galaxy 3C353

We report X-ray imaging of the powerful FR II radio galaxy 3C 353 using the Chandra X-ray Observatory. 3C 353's two 4-inch wide and 2-feet long jets allow us to study in detail the internal structure of the large-scale relativistic outflows at both radio and X-ray photon energies with the sub-arcsecond spatial resolution provided by the VLA and Chandra instruments. In a 90 ks Chandra observation, we have detected X-ray emission from most radio structures in 3C 353, including the nucleus, the jet and the counterjet, the terminal jet regions (hotspots), and one radio lobe. We show that the detection of the X-ray emission associated with the radio knots and counterknots, which is most likely non-thermal in origin, puts several crucial constraints on the X-ray emission mechanisms in powerful large-scale jets of quasars and FR II sources. In particular, we show that this detection is inconsistent with the inverse-Compton model proposed in the literature, and instead implies a synchrotron origin of the X-ray jet photons. We also find that the width of the X-ray counterjet is possibly narrower than that measured in radio bands, that the radio-to-X-ray flux ratio decreases systematically downstream along the jets, and that there are substantial …
Date: June 13, 2008
Creator: Kataoka, J.; Stawarz, L.; Harris, D.E.; Siemiginowska, A.; Ostrowski, M.; Swain, M.R. et al.
System: The UNT Digital Library
The work function of sub-monolayer cesium-covered gold: A photoelectronspectroscopy study (open access)

The work function of sub-monolayer cesium-covered gold: A photoelectronspectroscopy study

Using visible and X-ray photoelectron spectroscopy we measured the work function of a Au(111) surface at a well-defined sub-monolayer coverage of Cs. For a Cs coverage producing a photoemission maximum with a He-Ne laser, the work function is 1.61 {+-} 0.08 eV consistent with previous assumptions used to analyze vibrationally promoted electron emission. A discussion of possible Cs layer structures is also presented.
Date: June 13, 2008
Creator: LaRue, J. L.; White, J. D.; Nahler, N. H.; Liu, Z.; Sun, Y.; Pianetta, P. A. et al.
System: The UNT Digital Library
The US Support Program to IAEA Safeguards Priority of Training and Human Resources (open access)

The US Support Program to IAEA Safeguards Priority of Training and Human Resources

The U.S. Support Program to IAEA Safeguards (USSP) priority of training and human resources is aimed at providing the Department of Safeguards with an appropriate mixture of regular staff and extrabudgetary experts who are qualified to meet the IAEA's technical needs and to provide personnel with appropriate instruction to improve the technical basis and specific skills needed to perform their job functions. The equipment and methods used in inspection activities are unique, complex, and evolving. New and experienced safeguards inspectors need timely and effective training to perform required tasks and to learn new skills prescribed by new safeguards policies or agreements. The role of the inspector has changed from that of strictly an accountant to include that of a detective. New safeguards procedures are being instituted, and therefore, experienced inspectors must be educated on these new procedures. The USSP also recognizes the need for training safeguards support staff, particularly those who maintain and service safeguards equipment (SGTS), and those who perform information collection and analysis (SGIM). The USSP is committed to supporting the IAEA with training to ensure the effectiveness of all staff members and will continue to offer its assistance in the development and delivery of basic, refresher, and …
Date: June 13, 2008
Creator: Queirolo,A.
System: The UNT Digital Library
Measurements of the asymmetric, dynamic sheath around a pulse biased sphere immersed in flowing metal plasma (open access)

Measurements of the asymmetric, dynamic sheath around a pulse biased sphere immersed in flowing metal plasma

A long-probe technique was utilized to record the expansion and retreat of the dynamic sheath around a spherical substrate immersed in pulsed cathode arc metal plasma. Positively biased, long cylindrical probes were placed on the side and downstream of a negatively pulsed biased stainless steel sphere of 1" (25.4 mm) diameter. The amplitude and width of the negative high voltage pulses (HVP) were 2 kV, 5 kV, 10 kV, and 2 mu s, 4 mu s, 10 mu s, respectively. The variation of the probe (electron) current during the HVP is a direct measure for the sheath expansion and retreat. Maximum sheath sizes were determined for the different parameters of the HVP. The expected rarefaction zone behind the biased sphere (wake) due to the fast plasma flow was clearly established and quantified.
Date: June 13, 2008
Creator: Anders, Andre; Wu, Hongchen & Anders, Andre
System: The UNT Digital Library
Multivariate Clustering of Large-Scale Scientific Simulation Data (open access)

Multivariate Clustering of Large-Scale Scientific Simulation Data

Simulations of complex scientific phenomena involve the execution of massively parallel computer programs. These simulation programs generate large-scale data sets over the spatio-temporal space. Modeling such massive data sets is an essential step in helping scientists discover new information from their computer simulations. In this paper, we present a simple but effective multivariate clustering algorithm for large-scale scientific simulation data sets. Our algorithm utilizes the cosine similarity measure to cluster the field variables in a data set. Field variables include all variables except the spatial (x, y, z) and temporal (time) variables. The exclusion of the spatial dimensions is important since ''similar'' characteristics could be located (spatially) far from each other. To scale our multivariate clustering algorithm for large-scale data sets, we take advantage of the geometrical properties of the cosine similarity measure. This allows us to reduce the modeling time from O(n{sup 2}) to O(n x g(f(u))), where n is the number of data points, f(u) is a function of the user-defined clustering threshold, and g(f(u)) is the number of data points satisfying f(u). We show that on average g(f(u)) is much less than n. Finally, even though spatial variables do not play a role in building clusters, it …
Date: June 13, 2003
Creator: Eliassi-Rad, T & Critchlow, T
System: The UNT Digital Library
Qualification of Safety-Related Software in Nuclear Power Plants (open access)

Qualification of Safety-Related Software in Nuclear Power Plants

Digital instrumentation and control systems have the potential of offering significant benefits over traditional analog systems in Nuclear Power Plant safety systems, but there are also significant difficulties in qualifying digital systems to the satisfaction of regulators. Digital systems differ in fundamental ways from analog systems. New methods for safety qualification, which take these differences into account, would ease the regulatory cost and promote use of digital systems. This paper offers a possible method for assisting in the analysis of digital system software, as one step in an improved qualification process.
Date: June 13, 2000
Creator: Johnson, G L
System: The UNT Digital Library
''The Incubation Period for Void Swelling and its Dependence on Temperature, Dose Rate, and Dislocation Structure Evolution'' (open access)

''The Incubation Period for Void Swelling and its Dependence on Temperature, Dose Rate, and Dislocation Structure Evolution''

Void swelling in structural materials used for nuclear reactors is characterized by an incubation period whose duration largely determines the usefulness of the material for core components. Significant evolution of the dislocation and void microstructures that control radiation-induced swelling can occur during this period. Thus, a theory of incubation must treat time-dependent void nucleation in combination with dislocation evolution, in which the sink strengths of voids and dislocations change in concert. We present theoretical results for void nucleation and growth including the time-dependent, self-consistent coupling of point defect concentrations to the evolution of both void populations and dislocation density. Simulations show that the incubation radiation dose is a strong function of the starting dislocation density and of the dislocation bias factors for vacancy and interstitial absorption. Irradiation dose rate and temperature also affect the duration of incubation. The results are in general agreement with experiment for high purity metals.
Date: June 13, 2002
Creator: Surh, M. P.; Sturgeon, J. B. & Wolfer, W. G.
System: The UNT Digital Library
Calculation of Neutral Beam Injection into SSPX (open access)

Calculation of Neutral Beam Injection into SSPX

The SSPX spheromak experiment has achieved electron temperatures of 350eV and confinement consistent with closed magnetic surfaces. In addition, there is evidence that the experiment may be up against an operational beta limit for Ohmic heating. To test this barrier, there are firm plans to add two 0.9MW Neutral Beam (NB) sources to the experiment. A question is whether the limit is due to instability. Since the deposited Ohmic power in the core is relatively small the additional power from the beams is sufficient to significantly increase the electron temperature. Here we present results of computations that will support this contention. We have developed a new NB module to calculate the orbits of the injected fast fast-ions. The previous computation made heavy use of tokamak ordering which fails for a tight-aspect-ratio device, where B{sub tor} {approx} B{sub pol}. The model calculates the deposition from the NFREYA package [1]. The neutral from the CX deposition is assumed to be ionized in place, a high-density approximation. The fast ions are then assumed to fill a constant angular momentum orbit. And finally, the fast ions immediately assume the form of a dragged down distribution. Transfer rates are then calculated from this distribution function …
Date: June 13, 2006
Creator: Pearlstein, L. D.; Casper, T. A.; Hill, D. N.; LoDestro, L. L. & McLean, H. S.
System: The UNT Digital Library
Support for Whole-Program Analysis and the Verification of the One-Definition Rule in C++ (open access)

Support for Whole-Program Analysis and the Verification of the One-Definition Rule in C++

We present a compact and accurate representation of a whole-program abstract syntax tree, and use it to detect a specific security vulnerability in C++ programs known as a One-Definition Rule (ODR) violation. The ODR states that types and functions appearing in multiple compilation units must be defined identically. However, no current compiler can enforce ODR because doing so requires the ability to see the full application source at once; where ODR is violated, the program is incorrect. Moreover, a lack of ODR enforcement makes a program vulnerable to the so-called VPTR exploit, in which an object's virtual function table is replaced by malicious code. Our representation of the whole program preserves all features of the source for analysis and transformation, and permits a million-line application to fit entirely in the memory of a workstation with 1 GB of RAM.
Date: June 13, 2006
Creator: Quinlan, D; Vuduc, R; Panas, T; Haerdtlein, J & Saebjoernsen, A
System: The UNT Digital Library
Radiative b to d Penguins (open access)

Radiative b to d Penguins

This article gives an overview of the recent searches and measurements of b {yields} d penguin transitions with the BaBar experiment. The branching fraction of these decays in the Standard Model (SM) is expected to be a factor of 10 or more lower than the corresponding b {yields} s penguin transitions, but a deviation from the SM prediction would be an equally striking sign of new physics. The exclusive decay B {yields} {pi}{ell}{ell} is searched by BaBar with no excess over the background found. The BaBar measurement of B {yields} ({rho}, {omega}){gamma} provides the first evidence of B{sup +} {yields} {rho}{sup +}{gamma}, {sup c} is in good agreement with the previous Belle results and provides a measurement of |V{sub td}/V{sub ts}| independent of the one from Bs mixing. No deviation from the SM is found.
Date: June 13, 2007
Creator: Bechtle, P.
System: The UNT Digital Library
A Well-Defined, Silica-Supported Tungsten Imido Alkylidene OlefinMetathesis Catalyst (open access)

A Well-Defined, Silica-Supported Tungsten Imido Alkylidene OlefinMetathesis Catalyst

The reaction of [W(=NAr)(=CHtBu)(CH2tBu)2](1; Ar =2,6-iPrC6H3) with a silica partially dehydroxylated at 700oC, SiO2-(700),gives syn-[(_SiO)W(=NAr)(=CHtBu)(CH2tBu)](2) as a major surface species,which was fully characterized by mass balance analysis, IR, NMR, EXAFS,and DFT periodic calculations. Similarly, complex 1 reacts with[(c-C5H9)7Si7O12SiOH]to give [(SiO)W(=NAr)(=CHtBu)(CH2tBu)](2m), whichshows similar spectroscopic properties. Surface complex 2 is a highlyactive propene metathesis catalyst, which can achieve a TON of 16000within 100 h, with only a slow deactivation.
Date: June 13, 2006
Creator: Rhers, Bochra; Salameh, Alain; Baudouin, Anne; Quadrelli, ElsjeA.; Taoufik, Mostafa; Coperet, Christophe et al.
System: The UNT Digital Library
Photometric Redshifts in the IRAC Shallow Survey (open access)

Photometric Redshifts in the IRAC Shallow Survey

Accurate photometric redshifts are calculated for nearly 200,000 galaxies to a 4.5 micron flux limit of {approx} 13 {micro}Jy in the 8.5 deg{sup 2} Spitzer/IRAC Shallow survey. Using a hybrid photometric redshift algorithm incorporating both neural-net and template-fitting techniques, calibrated with over 15,000 spectroscopic redshifts, a redshift accuracy of {sigma} = 0.06 (1+z) is achieved for 95% of galaxies at 0 < z < 1.5. The accuracy is {sigma} = 0.12 (1 + z) for 95% of AGN at 0 < z < 3. Redshift probability functions, central to several ongoing studies of the galaxy population, are computed for the full sample. We demonstrate that these functions accurately represent the true redshift probability density, allowing the calculation of valid confidence intervals for all objects. These probability functions have already been used to successfully identify a population of Spitzer-selected high redshift (z > 1) galaxy clusters. We present one such spectroscopically confirmed cluster at <z> = 1.24, ISCS J1434.2+3426. Finally, we present a measurement of the 4.5 {micro}m-selected galaxy redshift distribution.
Date: June 13, 2006
Creator: Brodwin, M.; Brown, M.; Ashby, M.; Bian, C.; Brand, K.; Dey, A. et al.
System: The UNT Digital Library
Nonlinear Bayesian Algorithms for Gas Plume Detection and Estimation from Hyper-spectral Thermal Image Data (open access)

Nonlinear Bayesian Algorithms for Gas Plume Detection and Estimation from Hyper-spectral Thermal Image Data

This paper presents a nonlinear Bayesian regression algorithm for the purpose of detecting and estimating gas plume content from hyper-spectral data. Remote sensing data, by its very nature, is collected under less controlled conditions than laboratory data. As a result, the physics-based model that is used to describe the relationship between the observed remotesensing spectra, and the terrestrial (or atmospheric) parameters that we desire to estimate, is typically littered with many unknown "nuisance" parameters (parameters that we are not interested in estimating, but also appear in the model). Bayesian methods are well-suited for this context as they automatically incorporate the uncertainties associated with all nuisance parameters into the error estimates of the parameters of interest. The nonlinear Bayesian regression methodology is illustrated on realistic simulated data from a three-layer model for longwave infrared (LWIR) measurements from a passive instrument. This shows that this approach should permit more accurate estimation as well as a more reasonable description of estimate uncertainty.
Date: June 13, 2007
Creator: Heasler, Patrick G.; Posse, Christian; Hylden, Jeff L. & Anderson, Kevin K.
System: The UNT Digital Library
SHOCK INITIATION EXPERIMENTS AND MODELING OF COMPOSITION B AND C-4 (open access)

SHOCK INITIATION EXPERIMENTS AND MODELING OF COMPOSITION B AND C-4

Shock initiation experiments on the explosives Composition B and C-4 were performed to obtain in-situ pressure gauge data for the purpose of determining the Ignition and Growth reactive flow model with proper modeling parameters. A 101 mm diameter propellant driven gas gun was utilized to initiate the explosive charges containing manganin piezoresistive pressure gauge packages embedded in the explosive sample. Experimental data provided new information on the shock velocity versus particle velocity relationship for each of the investigated materials in their respective pressure range. The run-distance-to-detonation points on the Pop-plot for these experiments showed agreement with previously published data, and Ignition and Growth modeling calculations resulted in a good fit to the experimental data. These experimental data were used to determine Ignition and Growth reactive flow model parameters for these explosives. Identical ignition and growth reaction rate parameters were used for C-4 and Composition B, and the Composition B model also included a third reaction rate to simulate the completion of reaction by the TNT component. The Composition B model was then tested on existing short pulse duration, gap test, and projectile impact shock initiation with good results. This Composition B model can be applied to shock initiation scenarios that …
Date: June 13, 2006
Creator: Urtiew, P A; Vandersall, K S; Tarver, C M; Garcia, F & Forbes, J W
System: The UNT Digital Library
RECENT STUDIES OF URANIUM AND PLUTONIUM CHEMISTRY IN ALKALINE RADIOACTIVE WASTE SOLUTIONS (open access)

RECENT STUDIES OF URANIUM AND PLUTONIUM CHEMISTRY IN ALKALINE RADIOACTIVE WASTE SOLUTIONS

Solubility studies of uranium and plutonium in a caustic, radioactive Savannah River Site tank waste solution revealed the existence of uranium supersaturation in the as-received sample. Comparison of the results to predictions generated from previously published models for solubility in these waste types revealed that the U model poorly predicts solubility while Pu model predictions are quite consistent with experimental observations. Separate studies using simulated Savannah River Site evaporator feed solution revealed that the known formation of sodium aluminosilicate solids in waste evaporators can promote rapid precipitation of uranium from supersaturated solutions.
Date: June 13, 2006
Creator: King, W; Bill Wilmarth, B; David Hobbs, D & Tommy Edwards, T
System: The UNT Digital Library