PNNL conducted independent site evaluations for four sites at Fort Lewis, Washington, to determine their suitability for closure on behalf of the installation. These sites were recommended for "No Further Action" by previous invesitgators and included the Storm Water Outfalls/Industrial Waste Water Treatment Plant (IWTP), the Pesticide Rinse Area, the Old Fire Fighting Training Pit, and the Illicit PCB Dump Site.

A technique is proposed to generate electron beam with ultralow transverse emittance through laser assisted transverse-to-longitudinal emittance exchange. In the scheme a laser operating in the TEM10 mode is used to interact with the electron beam in a dispersive region and to initiate the emittance exchange. It is shown that with the proposed technique one can significantly downsize an x-ray free electron laser (FEL), which may greatly extend the availability of these light sources. A hard x-ray FEL operating at 1.5 {angstrom} with a saturation length within 30 meters using a 3.8 GeV electron beam is shown to be practically feasible.

Samples of four formulations of ethylene-propylene diene monomer (EPDM) elastomer were exposed to initially pure tritium gas at one atmosphere and ambient temperature for various times up to about 420 days in closed containers. Two formulations were carbon-black-filled commercial formulations, and two were the equivalent formulations without filler synthesized for this work. Tritium effects on the samples were characterized by measuring the sample volume, mass, flexibility, and dynamic mechanical properties and by noting changes in appearance. The glass transition temperature was determined by analysis of the dynamic mechanical properties. The glass transition temperature increased significantly with tritium exposure, and the unfilled formulations ceased to behave as elastomers after the longest tritium exposure. The filled formulations were more resistant to tritium exposure. Tritium exposure made all samples significantly stiffer and therefore much less able to form a reliable seal when employed as O-rings. No consistent change of volume or density was observed; there was a systematic lowering of sample mass with tritium exposure. In addition, the significant radiolytic production of gas, mainly protium (H{sub 2}) and HT, by the samples when exposed to tritium was characterized by measuring total pressure in the container at the end of each exposure and by …

We propose and analyze a scheme to achieve a seeded hard x-ray source based on a two-stage echo-enabled harmonic generation (EEHG) FEL. In the scheme an 180 nm seed laser covering the whole bunch is first used to modulate the beam when beam energy is 2 GeV. After passing through a strong chicane complicated fine structures are introduced into the phase space. The beam is again modulated by a short 180 nm laser that only interacts with the rear part of the beam and accelerated to 6 GeV. A chicane is then used to convert the energy modulation imparted to the rear part of the beam into density modulation. The density-modulated beam is sent through a radiator to generate intense 6 nm radiation which will be used to interact with the front fresh part of the bunch. Finally we generate in the front part of the beam density modulation at the 1199th harmonic of the seed laser. We will discuss the issues related to the realization of the seeded hard x-ray FEL.

The Linac Coherent Light Source, LCLS, at the SLAC National Accelerator Laboratory, SNAL, is the first hard x-ray Free Electron Laser. The Undulator Controls Module, UCM, controls five cams and two translation stages that regulate the position of each of the 33 permanent undulator magnet segments within 10 microns. The UCM package, hardware and software, was designed and built by the Advanced Photon Source at Argonne. Important lessons were learned throughout the collaborative design, installation, testing, and commissioning periods that could be invaluable to future similar controls projects.

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Carbonaceous particles are a minor constituent of the atmosphere but have a profound effect on air quality, human health, visibility and climate. The importance of carbonaceous particles has been increasingly recognized and become a mainstream topic at numerous conferences. Such was not the case in 1978, when the 1st International Conference on Carbonaceous Particles in the Atmosphere (ICCPA), or ''Carbon Conference'' as it is widely known, was introduced as a new forum to bring together scientists who were just beginning to reveal the importance and complexity of carbonaceous particles in the environment. Table 1 lists the conference dates, venues in the series as well as the proceedings, and special issues resulting form the meetings. Penner and Novakov (Penner and Novakov, 1996) provide an excellent historical perspective to the early ICCPA Conferences. Thirty years later, the ninth in this conference series was held at its inception site, Berkeley, California, attended by 160 scientists from 31 countries, and featuring both new and old themes in 49 oral and 83 poster presentations. Topics covered such areas as historical trends in black carbon aerosol, ambient concentrations, analytic techniques, secondary aerosol formation, biogenic, biomass, and HULIS1 characterization, optical properties, and regional and global climate effects. …

This report summarizes the research performed on the LDRD project 02-ERD-071 to develop a quantum-limited microwave amplifier based on a dc Superconducting Quantum Interference Device (dc-SQUID). This project began in June 2002 and concluded in May 2005. This project produced the lowest noise temperature amplifiers ever produced, both in absolute terms and in relation to the Standard Quantum Limit. Being an order of magnitude lower in noise than the best HFET devices available, they are of great interest to a number of groups. Potential applications are numerous, from dark-matter searches to national security applications in Quantum Information Processing. Collaborations started during this project are continuing with the goal of single-spin detection using the rf-SET. Publications are forthcoming covering both the experimental results and the theoretical modeling. The most important publication with the noise temperature results will appear after the low frequency follow-up experiment. The other publications in production cover the input impedance measurements and the resulting transmission line models.

A magnetically coupled microbalance system has been used to measure adsorption and desorption isotherms and rates of desorption for carbon tetrachloride on dry prepared porous silica particles with narrow pore size distributions in the mesoporous range. Pore size distributions estimated from the carbon tetrachloride isotherms were found to be in close agreement with those determined using standard low temperature nitrogen adsorption. Three different types of particles were studied, with average pore diameters of 2.7 nm, 4.6 nm, and 5.9 nm. Prior to desorption rate studies, evacuated particulate samples were charged with volatile organic vapor at pressures sufficient to fill all mesopores with condensed fluid. Desorption rates into dry flowing helium were determined at 25 °C and atmospheric pressure, using the microbalance system combined with chromatographic analysis of the exit helium stream. Initial rates were found to decrease significantly, as mass adsorbed decreased. This residual mass was desorbing at such a low rate, that it can be considered a migration resistant fraction of the original mass adsorbed. Attempts to remove this residual mass at higher temperatures were partially successful; however, differences between the microbalance and gas chromatograph responses leave open uncertainty about whether the residual mass was pure carbon tetrachloride. To …

Early projections of the Sludge Batch 4 (SB4) composition predicted relatively high concentrations of alumina (Al{sub 2}O{sub 3}, 23.5 wt%) and sulfate (SO{sub 4}{sup 2-}, 1.2 wt%) in the sludge. A high concentration of Al{sub 2}O{sub 3} in the sludge, combined with Na{sub 2}O additions in the frit, raises the potential for nepheline crystallization in the glass. However, strategic frit development efforts at the Savannah River National Laboratory (SRNL) have shown that frits containing a relatively high concentration of B{sub 2}O{sub 3} can both suppress nepheline crystallization and improve melt rates. A high sulfate concentration is a concern to the DWPF as it can lead to the formation of sulfate inclusions in the glass and/or the formation of a molten, sulfate-rich phase atop the melt pool. To avoid these issues, a sulfate concentration limit of 0.4 wt% SO{sub 4}{sup 2-} in glass was originally set in the Product Composition Control System (PCCS) used at DWPF. It was later shown that this limit could be increased to 0.6 wt% SO{sub 4}{sup 2-} in glass for the Frit 418, Sludge Batch 3 (SB3) system.

This report is a summary of socioeconomic data analyses conducted in support of the Radiological Monitoring Program during fiscal year 2001. Socioeconomic data contained in this report include estimates for the years 2000 and 2001 of the resident population in the vicinity of Yucca Mountain. The estimates presented in this report are based on selected Census 2000 statistics, and housing and population data that were acquired and developed in accordance with LP-RS-00 1 Q-M&0, Scientific Investigation of Economic, Demographic, and Agricultural Characteristics in the Vicinity of Yucca Mountain. The study area from which data were collected is delineated by a radial grid, consisting of 160 grid cells, that is suitable for evaluating the pathways and potential impacts of a release of radioactive materials to the environment within a distance of 84 kilometers from Yucca Mountain. Data are presented in a tabular format by the county, state, area, and grid cell in which housing units, households, and resident population are located. Also included is a visual representation of the distribution of the 2000 residential populations within the study area, showing Census 2000 geography, county boundaries, and taxing district boundaries for selected communities.

The harmonic generation process in a harmonic cascade (HC) FEL is subject to noise degradation which is proportional to the square of the total harmonic order. In this paper, we study the shot noise evolution in the first-stage modulator and radiator of a HC FEL that produces the dominant noise contributions. We derive the effective input noise for a modulator operating in the low-gain regime, and analyze the radiator noise for a density-modulated beam. The significance of these noise sources in different harmonic cascade designs is also discussed.

The principal goal of this project was to assess the molecular nature and stability of radionuclide (137-Cs, 90-Sr, and 129-I) immobilization during weathering reactions in bulk Hanford sediments and their high surface area clay mineral constituents. We focused on the unique aqueous geochemical conditions that are representative of waste-impacted locations in the Hanford site vadose zone: high ionic strength, high pH and high Al concentrations. The specific objectives of the work were to (i) measure the coupling of clay mineral weathering and contaminant uptake kinetics of Cs+, Sr2+ and I-; (ii) determine the molecular structure of contaminant binding sites and their change with weathering time during and after exposure to synthetic tank waste leachate (STWL); (iii) establish the stability of neoformed weathering products and their sequestered contaminants upon exposure of the solids to more “natural” soil solutions (i.e., after removal of the caustic waste source); and (iv) integrate macroscopic, microscopic and spectroscopic data to distinguish labile from non-labile contaminant binding environments, including their dependence on system composition and weathering time. During this funding period, we completed a large set of bench-scale collaborative experiments and product characterization aimed at elucidating the coupling between mineral transformation reactions and contaminant sequestration/stabilization. Our experiments …

Electron cloud instabilities in the Los Alamos ProtonStorage Ring (PSR) and those foreseen forthe Oak Ridge SpallationNeutron Source (SNS) are examined theoretically, numerically, andexperimentally.

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Although significant progress has been achieved in understanding the genetic and biochemical bases of the spore germination process, the structural basis for breaking the dormant spore state remains poorly understood. We have used atomic force microscopy (AFM) to probe the high-resolution structural dynamics of single Bacillus atrophaeus spores germinating under native conditions. Here we show that AFM can reveal previously unrecognized germination-induced alterations in spore coat architecture and topology as well as the disassembly of outer spore coat rodlet structures. These results and previous studies in other microorganisms suggest that the spore coat rodlets are structurally similar to amyloid fibrils. AFM analysis of the nascent surface of the emerging germ cell revealed a porous network of peptidoglycan fibers. The results are consistent with a honeycomb model structure for synthetic peptidoglycan oligomers determined by nuclear magnetic resonance. AFM is a promising experimental tool for investigating the morphogenesis of spore germination and cell wall peptidoglycan structure.

A salt solution (doped with Tc-99), that simulates the salt waste stream to be processed at the Saltstone Production Facility, was immobilized in grout waste forms with and without (1) ground granulated blast furnace slag and (2) pretreatment with iron salts. The degree of immobilization of Tc-99 was measured through monolithic and crushed grout leaching tests. Although Fe (+2) was shown to be effective in reducing Tc-99 to the +4 state, the strong reducing nature of the blast furnace slag present in the grout formulation dominated the reduction of Tc-99 in the cured grouts. An effective diffusion coefficient of 4.75 x 10{sup -12} (Leach Index of 11.4) was measured using the ANSI/ANS-16.1 protocol. The leaching results show that, even in the presence of a concentrated salt solution, blast furnace slag can effectively reduce pertechnetate to the immobile +4 oxidation state. The measured diffusivity was introduced into a flow and transport model (PORFLOW) to calculate the release of Tc-99 from a Saltstone Vault as a function of hydraulic conductivity of the matrix.

A manual for supervisory personnel to aid in formulating detailed instructions for operators and foremen employed in a green salt plant is given. A description of the processsteps in plant operation is contained. (C.J.G.)

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Our goal (see Project Objectives) is to deliver a dosimetry system which will enable both a Pu body burden of 0.3 kBq, and a 30 cGy {gamma} ray dose, to be separately estimated with a confidence limit of {+-}30%. In terms of the numbers analyzed and the data we have accrued, we have direct quantitative evidence that we are on track to providing such a comprehensive independent dosimetry system for Mayak workers. We had previously demonstrated that intra-chromosomal aberrations measured in peripheral blood lymphocytes can be used as a sensitive long-lived low-background quantitative biomarker of densely-ionizing radiation dose in individuals exposed many years ago. We propose to calibrate the system such that it can be used to estimate both the densely-ionizing internal plutonium exposure and the sparsely-ionizing external exposure in Mayak workers exposed to different combinations of these over a prolonged period, mostly many years ago. Our objective is to deliver a dosimetry system (set of calibration parameters) which will enable both a comparatively low Pu body burden of 0.3 kBq, and a comparatively low 30 cGy {gamma} ray dose (one of these or both of these) to be estimated with a confidence limit of {+-}30% (higher doses will of …

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The U.S. Department of Energy’s (DOE) commitment to assuring the health and safety of its workers includes the conduct of epidemiologic surveillance activities that provide an early warning system for health problems among workers. The Illness and Injury Surveillance Program monitors illnesses and health conditions that result in an absence of workdays, occupational injuries and illnesses, and disabilities and deaths among current workers.

This note presents constraints on Standard Model parameters using published and preliminary precision electroweak results measured at the electron-positron colliders LEP and SLC. The results are compared with precise electroweak measurements from other experiments, notably CDF and D0 at the Tevatron. Constraints on the input parameters of the Standard Model are derived from the combined set of results obtained in high-Q{sup 2} interactions, and used to predict results in low-Q{sup 2} experiments, such as atomic parity violation, Moeller scattering, and neutrino-nucleon scattering. The main changes with respect to the experimental results presented in 2008 are new combinations of results on the W-boson mass and the mass of the top quark.

The U.S. Department of Energy’s (DOE’s) Building Energy Codes Program (BECP) has been asked by some states and energy code stakeholders to address the comparability of the 2009 International Energy Conservation Code® (IECC) as applied to commercial buildings and ANSI/ASHRAE/IESNA Standard 90.1-2007 (hereinafter referred to as Standard 90.1-07). An assessment of comparability will help states respond to and implement conditions specified in the State Energy Program (SEP) Formula Grants American Recovery and Reinvestment Act Funding Opportunity, Number DE-FOA-0000052, and eliminate the need for the states individually or collectively to perform comparative studies of the 2009 IECC and Standard 90.1-07. The funding opportunity announcement contains the following conditions: (2) The State, or the applicable units of local government that have authority to adopt building codes, will implement the following: (A) A residential building energy code (or codes) that meets or exceeds the most recent International Energy Conservation Code, or achieves equivalent or greater energy savings. (B) A commercial building energy code (or codes) throughout the State that meets or exceeds the ANSI/ASHRAE/IESNA Standard 90.1-2007, or achieves equivalent or greater energy savings . (C) A plan to achieve 90 percent compliance with the above energy codes within eight years. This plan will …