Report discussing studies regarding properties of the zirconium-uranium epsilon phase related to stability and existence range. Data showing this phase's thermodynamic stability is presented as well as the zirconium-uranium constitutional diagram. Oxygen and nitrogen effects on zirconium-uranium alloys and epsilon-phase alloys is included as well as ternary zirconium-uranium-oxygen diagrams.

Abstract: "Approximate melting points have been determined for five samples of uranium tetrafluoride representing incompletely converted uranium dioxide and covering the range from about 2 to 20 w/o UO2, using the method of differential thermal analysis. The results indicate the melting temperatures are in the range of 920 to 980 C. No significant correlation between melting point and UO2 content was observed, possibly because of calcite formation. Similar results were obtained on synthetic mistakes of UF4 containing from 10 to 40 w/o UO2."