IONIUM (THORIUM-230) FOR RADIOISOTOPE PREPARATION--STATUS REPORT (open access)

IONIUM (THORIUM-230) FOR RADIOISOTOPE PREPARATION--STATUS REPORT

The general prospects of several radioisotopes are reviewed; the special properties of U/sup 232/ and Th/sup 228/ are poi nted out; and ionium (Th/sup 230/ ) and protactinium target materials are discussed from the sthndpoint of availability and chemical separations processes required for the preparation of U/ sup 232/ and Th/sup 228/. Outlines are given for potential schem es for the separation of U/sup 232/ and Th/sup 228/ from uranium milling pr ocess waste streams and from the irradiation products of Th/sup 230/--Th/sup 232/ mixtures. The high heat generating rates of these potent alpha emitters make them especially suitable for primary consideration as heat sources for small thermoelectric generators. The exceptionally high alpha activity suggests their use in special neutron sources as Ra-Be sources, and they may have sufficiently high neutron generating rates to be in contention with some of the smaller research reactors and experimental neutron producers. (B.O.G.)
Date: December 15, 1959
Creator: Coppinger, E.A. & Rohrmann, C.A.
System: The UNT Digital Library
Preliminary Studies of Scavenging Systems Related to Radioactive Fallout. Letter Report No. 7 Covering Period April 1 to May 31, 1959 (open access)

Preliminary Studies of Scavenging Systems Related to Radioactive Fallout. Letter Report No. 7 Covering Period April 1 to May 31, 1959

Progress is reported on the development of a cyclone which will remove particles larger than 8 microns. A method is proposed for a more efficient separation of particles by increasing the number of size separation filters in the sampling train. Preliminary tests with submicron polystyrene particles are being conducted. Numerous methods have been tried for counting the particles in a water droplet of the polystyrene aerosol. The criteria for a satisfactory method of counting particles are discussed. A proposed method to accomplish this is to use carbon-14 labeled polystyrene hydrosols. (For preceding period see ARF-3127-6.) (B.O.G.)
Date: June 15, 1959
Creator: Stockham, J. D. & Rosinski, J.
System: The UNT Digital Library
The Early Antiproton Work [Nobel Lecture] (open access)

The Early Antiproton Work [Nobel Lecture]

Early work on the antiproton, particularly that part which led to the first paper on the subject, is described. Conclusions that can be drawn purely from the existence of the antiproton are discussed. (W.D.M.)
Date: December 15, 1959
Creator: Chamberlain, O.
System: The UNT Digital Library
PERFORMANCE TEST OF A TWO-COOLANT-REGION SODIUM PUMP SHAFT FREEZE-SEAL (open access)

PERFORMANCE TEST OF A TWO-COOLANT-REGION SODIUM PUMP SHAFT FREEZE-SEAL

The operation of the freeze-seal type sodium pump requires a shaft freeze-seal capable of retaining sodium. A prototype two-coolant-region freeze seal for application on HNPF sodium pumps was designed and constructed. It was tested under environmental conditions to determine its operating characteristics and sodium retaining capabilities. (auth)
Date: July 15, 1959
Creator: Streck, F.O.
System: The UNT Digital Library
THE CONTROL OF BERYLLIUM HAZARDS (open access)

THE CONTROL OF BERYLLIUM HAZARDS

The toxicological properties of beryllium and compounds of beryllium are briefly reviewed, together with the historical developmert of the recommendations for maximum permissible beryllium air concentrations. The application of the enclosure technique for the control of beryllium hazards is described. Emphasis is placed on the design objectives of partial and total enclosures and the related function of auxiliary components. Monitoring procedures used to evaluate the performance of enclosures are discussed. (auth)
Date: July 15, 1959
Creator: Lindeken, C. L. & Meadors, O. L.
System: The UNT Digital Library
GAMMA-RAY AND FAST NEUTRON ANNULAR STREAMING EVALUATION THROUGH SODIUM REACTOR EXPERIMENT (SRE)-MARK II CONTROL AND SAFETY ROD ASSEMBLIES (open access)

GAMMA-RAY AND FAST NEUTRON ANNULAR STREAMING EVALUATION THROUGH SODIUM REACTOR EXPERIMENT (SRE)-MARK II CONTROL AND SAFETY ROD ASSEMBLIES

An experimental program was initiated io determine the extent of fast neutron and gamma ray streaming through the SRL Mark II control and safety rods and to evaluate the adequacy of the shielding provided in these control and safety rods. The methods and procedures used to evaluate these problems are routine and proven for determining gamma-ray and fast neutron dosages using radiation sensitive films and gold foils. The final experimental results indicated that no excessive streaming of either gamma rays or fast neutrons is present above or around the SHE Mark II control and safety rods. The analytical attenuation methods used to calculate the fast neutron and gamma-ray streaming dose rates gave results that compared favorably with the experimental data. Even ihough the agreement was favorable, it cannot be concluded that these analyical methods would be equally valid for other annular geometries. Additional experimental work will be necessary in order to establish the validity for performing similar analysis, but the favorable agreement encourages the use of such methods until other methods are determined. (auth)
Date: October 15, 1959
Creator: Anderson, F. D.
System: The UNT Digital Library
HRT Process Flowsheets--Revised Edition (open access)

HRT Process Flowsheets--Revised Edition

Revised HRT flowsheets are presented. These revisions cover such items as relocation of freezer units on the lines, corrections to the numbering of lines, valves or instruments, and the addition of a few lines in the service areas. The waste and vent system flowsheet was redrawn as two sheets. (C.J.G.)
Date: December 15, 1959
Creator: Robertson, R. C. & Jones, J. E.
System: The UNT Digital Library
MEASUREMENT OF THE SRE AND KEWB PROMPT NEUTRON LIFETIME USING RANDOM NOISE AND REACTOR OSCILLATION TECHNIQUES (open access)

MEASUREMENT OF THE SRE AND KEWB PROMPT NEUTRON LIFETIME USING RANDOM NOISE AND REACTOR OSCILLATION TECHNIQUES

The prompt neutron lifetime of the SRE was measured by both the oscillation and random noise techniques. Measurement by use of the oscillation technique gave a prompt neutron lifetime of (5 25 plus or minus 0 35) x 10/sup - 4/ sec for a calculated beta of 7 x 10/sup -3/. The measured noise response indicated a lifetime of (5.25 plus or minus 0.7) x 10/sup -4/ sec. Both measured values are in agreement with the calculated value of 5 x 10/sup -4/ sec. Four experiments utilizing the noise analysis technique were performed to determine the prompt neutron lifetime of the KEWB. All four experiments gave results which agreed within 3%, For an estimated beta of 8 x 10/sup -3/, the measured value obtained was (7.8 plus or minus 0.3) x 10/sup -5/ sec. This is in reasonable agreement with both the energy independert calculated value of 6.6 x 10/sup -5/ see and the value of 6.2 x 10/sup -5/ sec obtained from the experimental inhour equation The oscillation technique has been found to be better suited for lifetime determinations in reactors where the prompt neutron break frequency is less than 5 cps. Reactor noise analysis is more suitable for …
Date: October 15, 1959
Creator: Griffin, C. W. & Lundholm Jr., J. G.
System: The UNT Digital Library
PATHFINDER ATOMIC POWER PLANT COOLANT DISTRIBUTION TESTS. Final Report (open access)

PATHFINDER ATOMIC POWER PLANT COOLANT DISTRIBUTION TESTS. Final Report

Tests were made to determine the head loss coefficient through the inlet plenum of the Pathfinder reactor and to determine the now distribution among the fuel element nozzles for various operating conditions--with all three pumps operating at the same flow rate and with any combination of only two pumps operating at the same flow rate. A quarter-scale wooden model was used for the tests. Air was used as the fluld. The loss coefficient was determined to be 1.8 plus or minus 0.3. The velocities of flow through the fuel element nozzles were determined to be within plus or minus 5 per cent of average flow when all pumps are operating and within plus or minus 10 per cent of average flow when only two pumps are operating. (auth)
Date: November 15, 1959
Creator: Wilson, J. & Styles, R.
System: The UNT Digital Library
Reprocessing of Low-Enrichment Uranium-Molybdenum Alloy Fuels (open access)

Reprocessing of Low-Enrichment Uranium-Molybdenum Alloy Fuels

Procedures for the dissolution of U-Mo alloy fuels to prepare feed solutions for low-acid (Redox) type solvent extraction processing are presented. U-Mo alloys can be dissolved in boiling ferric nitrate--ritric acid solutions to higher terminal urarium concentrations and lower terminal acidities without precipitation of uranyl molybdate than in nitric acid alone. Anion resin exchange studies indicate the presence of negatively charged iron-molybdenum complex ions in the solutions. The U-Mo alloys also dissolve more rapidly in ferric nitrate--nitnic acid solutions than in nitric acid alone; dissolution rate data are given. Curves delineating free acid, uranium, snd iron (III) concentrations within which solutions stable towards solids formation can be prepared from U-3 wt.% Mo and U-10 wt.% Mo alloys are presented. Stability during prolonged storage of uranium--molybdenum-ferric nitrate--nitric acid solutions is discussed. Data on the oxidation of plutonium in these solutions and on further neutralization of the solutions are presented. Fission product decontamination and product recovery obtained in solvent extraction studies simulating the Redox process are discussed. (auth)
Date: September 15, 1959
Creator: Schulz, W. W. & Duke, E. M.
System: The UNT Digital Library
Determination of Oxygen in Oxide Films by Neutron Activation Analysis (open access)

Determination of Oxygen in Oxide Films by Neutron Activation Analysis

Preliminary experiments were conducted to evaluate the use of the nuclear reactions Li/sup 6/ (n, alpha )H/sup 3/ and O/sup 16/(H/sup 3/,n) F/sup 18/ to determine the thickness of oxide films on metals. Sheets of thin paper and of aluminum, imbedded in powdered LiF, were irradiated with pile neutrons at a flux of 6 x 10/sup 11/ n/cm/sup 2//sec and counted with an end-window proportional counter. A saturation activity of 1.87 hr F/sup 18/ of 150 dis/min per microgram of oxygen was observed in the paper, but radioactivity due to impurities masked F/sup 18/ in the aluminum. It is concluded that a 1 A (0.01 mu gm/cm/sup 2/) oxide film thickness may be measured by a neutron irradiation at a flux of 10/sup 14/ n/cm/sup 2//sec but chemical separation of induced radioactivity from the bulk metal is essential. (auth)
Date: July 15, 1959
Creator: Winchester, J. W.; Meyer, R. E.; Bate, L. C. & Leddicotte, G. W.
System: The UNT Digital Library
Electrical Resistivity Data for Heat-Transfer Test-Section Metals (open access)

Electrical Resistivity Data for Heat-Transfer Test-Section Metals

Electrical resistivity data for metals which are likely to be resistance heated in heat-transfer tests were compiled and are given as a function of temperature. (auth)
Date: April 15, 1959
Creator: Gambill, W. R.
System: The UNT Digital Library