Improvisation is an art form which has arguably been present since the existence of music itself. Inventing music on the spot, like spontaneous speech, is a common expression of artistry throughout history and across musical boundaries. While improvisation has maintained its importance in jazz, classical organ music and the music of many eastern cultures, this dissertation will focus on the presence of improvisation as acceptable performance practice within the tradition of western classical music. At several points in history, this musical tradition was encouraged and even expected to be a regular part of a musician's life, and yet in the classical music tradition of the twenty-first century, improvisation is rarely, if ever, heard from the concert stage, nor is it regularly included in the general education of the conservatory student.

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This dissertation is devoted to the development of novel devices for optoelectronic and photovoltaic applications using the promise of inkjet printing with two-dimensional (2D) materials. A systematic approach toward the characterization of the liquid exfoliated 2D inks comprising of graphene, molybdenum disulfide (MoS2), tungsten diselenide (WSe2), and 2D perovskites is discussed at depth. In the first study, the biocompatibility of 2D materials -- graphene and MoS2 -- that were drop cast onto flexible PET and polyimide substrates using mouse embryonic fibroblast (STO) and human esophageal fibroblast (HEF) cell lines, was explored. The polyimide samples for both STO and HEF showed high biocompatibility with a cell survival rate of up to ~ 98% and a confluence rate of 70-98%. An inkjet printed, biocompatible, heterostructure photodetector was constructed using inks of photo-active MoS2 and electrically conducting graphene, which facilitated charge collection of the photocarriers. The importance of such devices stems from their potential utility in age-related-macular degeneration (AMD), which is a condition where the photosensitive retinal tissue degrades with aging, eventually compromising vision. The biocompatible inkjet printed 2D heterojunction devices were photoresponsive to broadband incoming radiation in the visible regime, and the photocurrent scaled proportionally with the incident light intensity, exhibiting a …