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Electrostatic Mechanism of Emission Enhancement in Hybrid Metal-semiconductor Light-emitting Heterostructures
III-V nitrides have been put to use in a variety of applications including laser diodes for modern DVD devices and for solid-state white lighting. Plasmonics has come to the foreground over the past decade as a means for increasing the internal quantum efficiency (IQE) of devices through resonant interaction with surface plasmons which exist at metal/dielectric interfaces. Increases in emission intensity of an order of magnitude have been previously reported using silver thin-films on InGaN/GaN MQWs. the dependence on resonant interaction between the plasmons and the light emitter limits the applications of plasmonics for light emission. This dissertation presents a new non-resonant mechanism based on electrostatic interaction of carriers with induced image charges in a nearby metallic nanoparticle. Enhancement similar in strength to that of plasmonics is observed, without the restrictions imposed upon resonant interactions. in this work we demonstrate several key features of this new interaction, including intensity-dependent saturation, increase in the radiative recombination lifetime, and strongly inhomogeneous light emission. We also present a model for the interaction based on the aforementioned image charge interactions. Also discussed are results of work done in the course of this research resulting in the development of a novel technique for strain measurement …
Date:
May 2012
Creator:
Llopis, Antonio
Object Type:
Thesis or Dissertation
System:
The UNT Digital Library
San Antonio Register (San Antonio, Tex.), Vol. 8, No. 14, Ed. 1 Friday, July 8, 1938
Weekly newspaper from San Antonio, Texas that includes local, state, and national news along with advertising.
Date:
July 8, 1938
Creator:
Andrews, U. J.
Object Type:
Newspaper
System:
The Portal to Texas History
San Antonio Express. (San Antonio, Tex.), Vol. 46, No. 295, Ed. 1 Sunday, October 22, 1911
Daily newspaper from San Antonio, Texas that includes local, state and national news along with advertising.
Date:
October 22, 1911
Creator:
unknown
Object Type:
Newspaper
System:
The Portal to Texas History
Metallic Nanodroplet Induced Coulomb Catalysis for Off-Resonant Plasmonic Enhancement of Photoemission in Semiconductors
This article reports a new mechanism based on electrostatic interactions of carriers and their image charges in metals to generate more photons from optical sources at frequencies that are off-resonant to the localized plasmon frequency.
Date:
April 8, 2016
Creator:
Neogi, Arup; Grycznski, Karol G.; Llopis, A.; Lin, Jie; Main, Kyle; Shimada, Ryoko et al.
Object Type:
Article
System:
The UNT Digital Library
La Prensa (San Antonio, Tex.), Vol. 4, No. 724, Ed. 1 Thursday, November 9, 1916
Daily Spanish-language newspaper from San Antonio, Texas that includes local, state, and national news along with advertising.
Date:
November 9, 1916
Creator:
Lozano, Ignacio E.
Object Type:
Newspaper
System:
The Portal to Texas History
Freie Presse für Texas. (San Antonio, Tex.), Vol. 29, No. 3685, Ed. 1 Friday, May 18, 1894
Daily German-language newspaper from San Antonio, Texas that includes local, state, and national news along with advertising.
Date:
May 18, 1894
Creator:
Hanschke, Robert
Object Type:
Newspaper
System:
The Portal to Texas History
Tri-Weekly Alamo Express. (San Antonio, Tex.), Vol. 1, No. 19, Ed. 1 Monday, March 18, 1861
Tri-weekly newspaper from San Antonio, Texas that includes local, state and national news along with advertising.
Date:
March 18, 1861
Creator:
Newcomb, J. P.
Object Type:
Newspaper
System:
The Portal to Texas History
Comprehensive Microfilm Index of Roll 31: Archivo del Convento de Santa Cruz de Queretaro Convento de San Francisco, Celaya
Compilation of forms that provide an overview of topics, names, and other content of original documents on microfilm at the Old Spanish Mission Historical Research Library.
Date:
February 1983
Creator:
Rock, Rosalind Z.
Object Type:
Text
System:
The Portal to Texas History
Ultrafast Spectroscopy of Hybrid Ingan/gan Quantum Wells
Group III nitrides are efficient light emitters. The modification of internal optoelectronic properties of these materials due to strain, external or internal electric field are an area of interest. Insertion of metal nanoparticles (MNPs) (Ag, Au etc) inside the V-shaped inverted hexagonal pits (IHP) of InGaN/GaN quantum wells (QWs) offers the potential of improving the light emission efficiencies. We have observed redshift and blueshift due to the Au MNPs and Ag MNPs respectively. This shift could be due to the electric field created by the MNPs through electrostatic image charge. We have studied the ultrafast carrier dynamics of carriers in hybrid InGaN/GaN QWs. The change in quantum confinement stark effect due to MNPs plays an important role for slow and fast carrier dynamics. We have also observed the image charge effect on the ultrafast differential transmission measurement due to the MNPs. We have studied the non-linear absorption spectroscopy of these materials. The QWs behave as a discharging of a nanocapacitor for the screening of the piezoelectric field due to the photo-excited carriers. We have separated out screening and excitonic bleaching components from the main differential absorption spectra of InGaN/GaN QWs.
Date:
August 2012
Creator:
Mahat, Meg Bahadur
Object Type:
Thesis or Dissertation
System:
The UNT Digital Library
Interaction of Plasmons and Excitons for Low-Dimension Semiconductors
The effects of surface plasmon for InGaN/GaN multi-quantum wells and ZnO nanoparticles optical linear and nonlinear emission efficiency had been experimentally studied. Due to the critical design for InGaN MQWs with inverted hexagonal pits based on GaN, both contribution of surface plasmon effect and image charge effect at resonant and off resonant frequencies were experimentally and theoretically investigated. With off- resonant condition, the InGaN MQWs emission significantly enhanced by metal nanoparticles. This enhancement was caused by the image charge effect, due to the accumulation of carriers to NPs region. When InGaN emission resonated with metal particles SP modes, surface Plasmon effect dominated the emission process. We also studied the surface plasmon effect for ZnO nanoparticles nonlinear optical processes, SHG and TPE. Defect level emission had more contribution at high incident intensity. Emissions are different for pumping deep into the bulk and near surface. A new assumption to increase the TPE efficiency was studied. We thought by using Au nanorods localized surface plasmon mode to couple the ZnO virtual state, the virtual state’s life time would be longer and experimentally lead the emission enhancement. We studied the TPE phenomena at high and near band gap energy. Both emission intensity and decay …
Date:
December 2014
Creator:
Lin, Jie (physicist)
Object Type:
Thesis or Dissertation
System:
The UNT Digital Library
[Commencement Program for University of North Texas, May 11-12, 2012]
Commencement program for the spring 2012 graduating class of the University of North Texas, held in the UNT Coliseum on Friday and Saturday, May 11-12, 2012. The program contains the order of service and a list of graduates for the baccalaureate, master's, doctoral degrees.
Date:
2012-05-11/2012-05-12
Creator:
University of North Texas
Object Type:
Pamphlet
System:
The UNT Digital Library
UNT Libraries Digital Infrastructure
This presentation discusses the digital infrastructure of the University of North Texas (UNT) Libraries. It gives a timeline of the UNT Libraries' digital projects with examples.
Date:
December 10, 2012
Creator:
Phillips, Mark Edward
Object Type:
Presentation
System:
The UNT Digital Library
The Informer and Texas Freeman (Houston, Tex.), Vol. 17, No. 8, Ed. 1 Saturday, August 17, 1935
Weekly African-American newspaper from Houston, Texas that includes local, state, and national news along with advertising.
Date:
August 17, 1935
Creator:
unknown
Object Type:
Newspaper
System:
The Portal to Texas History
The Houston Informer (Houston, Tex.), Vol. 7, No. 3, Ed. 1 Saturday, June 6, 1925
Weekly African-American newspaper from Houston, Texas that includes local, state, and national news along with advertising.
Date:
June 6, 1925
Creator:
Richardson, Clifton F.
Object Type:
Newspaper
System:
The Portal to Texas History
The Dallas Craftsman (Dallas, Tex.), Vol. 38, No. 18, Ed. 1 Friday, April 6, 1951
Weekly newspaper from Dallas, Texas that includes news and information concerning the labor movement along with advertising.
Date:
April 6, 1951
Creator:
Reilly, Wallace
Object Type:
Newspaper
System:
The Portal to Texas History
Particles, processes and materials for modern energy needs: Development of a DOE-EPSCoR project in Puerto Rico. Final report for September 30, 1997 - August 31, 2000
Twenty-eight (28) faculty researchers focused on High Energy Particle Physics, Novel Thin Film Materials for Optoelectronic Applications, and Catalytic Processes for Energy Sources and Environmental Detoxification to address problems cited as priorities by the DOE and local agencies. The High Energy Particle Physics cluster has DOE-competitive funding, and the number of cluster investigators who have competitive mainstream funding has increased from 2 to 13 since the inception of the program. In this reporting period, 8 postdoctorals, 38 graduate studnets, and 23 undergraduates were involved in DOE projects, and 191 publications and 238 presentations were generated. The UPR-Arecibo Integrated Science Multi-Use Laboratory provided workshops and other activities that directly impacted 360 teachers and 600 students and indirectly impacted over 25,000 through the enhancement of teachers' skills and knowledge.
Date:
September 29, 2000
Creator:
Weiner, Brad R.
Object Type:
Report
System:
The UNT Digital Library
Southwest Retort, Volume 74, Number 8, April 2022
This publication of the Dallas-Fort Worth Section of the American Chemical Society includes information about research, prominent scientist, organizational business, and various other stories of interest to the community.
Date:
April 2022
Creator:
American Chemical Society. Dallas/Fort Worth Section.
Object Type:
Journal/Magazine/Newsletter
System:
The UNT Digital Library
The Houston Informer (Houston, Tex.), Vol. 8, No. 28, Ed. 1 Saturday, November 27, 1926
Weekly African-American newspaper from Houston, Texas that includes local, state, and national news along with advertising.
Date:
November 27, 1926
Creator:
Richardson, Clifton F.
Object Type:
Newspaper
System:
The Portal to Texas History
The Houston Informer (Houston, Tex.), Vol. 8, No. 14, Ed. 1 Saturday, August 21, 1926
Weekly African-American newspaper from Houston, Texas that includes local, state, and national news along with advertising.
Date:
August 21, 1926
Creator:
Richardson, Clifton F.
Object Type:
Newspaper
System:
The Portal to Texas History
Věstník (West, Tex.), Vol. 21, No. 12, Ed. 1 Wednesday, February 1, 1933
Weekly Czech language newspaper from West, Texas published as the official organ of the Slavonic Benevolent Order of the State of Texas that includes news of interest to members, and local, state and national news along with advertising.
Date:
February 1, 1933
Creator:
Moučka, Franta
Object Type:
Newspaper
System:
The Portal to Texas History
Yoakum Daily Herald (Yoakum, Tex.), Vol. 33, No. 229, Ed. 1 Monday, December 30, 1929
Daily newspaper from Yoakum, Texas that includes local, state and national news along with extensive advertising.
Date:
December 30, 1929
Creator:
Morgan, Cena S.
Object Type:
Newspaper
System:
The Portal to Texas History
Mt. Pleasant Daily Times (Mount Pleasant, Tex.), Vol. 28, No. 245, Ed. 1 Wednesday, February 5, 1947
Daily newspaper from Mount Pleasant, Texas that includes local, state, and national news along with advertising.
Date:
February 5, 1947
Creator:
Cross, G. W.
Object Type:
Newspaper
System:
The Portal to Texas History
The Bryan Daily Eagle and Pilot (Bryan, Tex.), Vol. 29, No. 256, Ed. 1 Saturday, October 24, 1914
Daily newspaper from Bryan, Texas that includes local, state, and national news along with advertising.
Date:
October 24, 1914
Creator:
Buchanan, A. J.
Object Type:
Newspaper
System:
The Portal to Texas History
The Cuero Record. (Cuero, Tex.), Vol. 41, No. 193, Ed. 1 Sunday, August 18, 1935
Daily newspaper from Cuero, Texas that includes local, state, and national news along with advertising.
Date:
August 18, 1935
Creator:
Howerton, J. C.
Object Type:
Newspaper
System:
The Portal to Texas History