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Crystal field interaction in the pyrochlore magnet Ho{sub 2}Ti{sub 2}O{sub 7}. (open access)

Crystal field interaction in the pyrochlore magnet Ho{sub 2}Ti{sub 2}O{sub 7}.

Neutron time-of-flight spectroscopy has been employed to study the crystal field interaction in the pyrochlore titanate Ho{sub 2}Ti{sub 2}O{sub 7}. The crystal field parameters and corresponding energy level scheme have been determined from a profile fit to the observed neutron spectra. The groundstate is a well separated E{sub g} doublet with a strong Ising like anisotropy, which can give rise to titration in the pyrochlore lattice. Using the crystal field parameters determined for the Ho compound as an estimate of the crystal field interaction in other pyrochlore magnets, we also find the Ising type behavior for Dy. In contrast, the almost planar like anisotropy found for Er and Yb prevents frustration, because of the continuous range of possible spin orientations in this case.
Date: September 30, 1999
Creator: Rosenkranz, S.; Ramirez, A. P.; Hayashi, A.; Cava, R. J.; Siddharthan, R. & Shastry, B. S.
System: The UNT Digital Library